A highly promising route to scale millions of qubits is to use quantum photonic integrated circuits (PICs), where deterministic photon sources, reconfigurable optical elements, and single-photon detectors are monolithically integrated on the same silicon chip. The isolation of single-photon emitters, such as the G centers and W centers, in the optical telecommunication O-band, has recently been realized in silicon. In all previous cases, however, single-photon emitters were created uncontrollably in random locations, preventing their scalability. Here, we report the controllable fabrication of single G and W centers in silicon wafers using focused ion beams (FIB) with high probability. We also implement a scalable, broad-beam implantation protocol compatible with the complementary-metal-oxide-semiconductor (CMOS) technology to fabricate single telecom emitters at desired positions on the nanoscale. Our findings unlock a clear and easily exploitable pathway for industrial-scale photonic quantum processors with technology nodes below 100 nm.
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http://dx.doi.org/10.1038/s41467-022-35051-5 | DOI Listing |
J Phys Chem A
December 2024
Department of Chemistry, Colorado State University, Fort Collins, Colorado 80523, United States.
Time-resolved single molecule localization microscopy (TR-SMLM) with a 2 × 2 pixel fiber optic array camera was combined with time-correlated single photon counting (TCSPC) to obtain super-resolved fluorescence lifetime images of individual Cy3 dye molecules and individual colloidal CdSe/CdS/ZnS core/shell/shell semiconductor quantum dots (QDs). The characteristic blinking and bleaching behavior of the Cy3 and the blinking behavior of the QD emitters were used as distinguishing optical characteristics to isolate them and determine their centroid locations with spatial resolution below the optical diffraction limit. TCSPC was used to characterize the fluorescence lifetime and intensity corresponding to each emitter location.
View Article and Find Full Text PDFAdv Mater
December 2024
Shaanxi Joint Lab of Graphene, State Key Lab Incubation Base of Photoelectric Technology and Functional Materials, International Collaborative Center on Photoelectric Technology and Nano Functional Materials, Institute of Photonics & Photon-Technology, Northwest University, Xi'an, 710069, P. R. China.
Bulk photovoltaic effect (BPVE) can break the Shockley-Queisser limit by leveraging the inherent asymmetry of crystal lattice without a junction. However, this effect is mainly confined to UV-vis spectrum due to the wide-bandgap nature of traditional ferroelectric materials, thereby limiting the exploration of the infrared light-driven efficient BPVE. Herein, giant two-photon absorption (TPA) driven BPVE is uncovered from visible to infrared in ferroelectric α-InSe utilizing wavelength-tunable terahertz (THz) emission spectroscopy.
View Article and Find Full Text PDFIn large-area quantum networks based on optical fibers, photons are the fundamental carriers of information as so-called flying qubits. They may also serve as the interconnect between different components of a hybrid architecture, which might comprise atomic and solid-state platforms operating at visible or near-infrared wavelengths, as well as optical links in the telecom band. Quantum frequency conversion is the pathway to change the color of a single photon while preserving its quantum state.
View Article and Find Full Text PDFJ Phys Condens Matter
December 2024
Solid State and Structural Chemistry Unit, Indian Institute of Science, Bangalore 560012, India.
Solution grown quantum dots (QD) are promising materials for photonic quantum science. These materials are strongly confined and further offer advantages in terms of customizability and scalability. In this review we describe the applications of these materials towards quantum science particularly as single photon emitters.
View Article and Find Full Text PDFACS Nano
December 2024
Technology Innovation Center of Materials and Devices for Extreme Environment, School of Materials Science and Engineering, Harbin Institute of Technology, Harbin 150001, China.
Defects in chemical vapor deposition (CVD)-grown monolayer MoS are unavoidable and provide a powerful approach to creating single-photon emitters and quantum information systems through localizing excitons. However, insight into the A trion and B/C exciton localization in monolayer MoS remains elusive. Here, we investigate defect-mediated A trion and B/C exciton localization and relaxation in CVD-grown monolayer MoS samples via transient absorption spectroscopy.
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