The building block of in-memory computing with spintronic devices is mainly based on the magnetic tunnel junction with perpendicular interfacial anisotropy (p-MTJ). The resulting asymmetric write and readout operations impose challenges in downscaling and direct cascadability of p-MTJ devices. Here, we propose that a previously unimplemented symmetric write and readout mechanism can be realized in perpendicular-anisotropy spin-orbit (PASO) quantum materials based on FeGeTe and WTe. We demonstrate that field-free and deterministic reversal of the perpendicular magnetization can be achieved using unconventional charge-to--spin conversion. The resulting magnetic state can be readily probed with its intrinsic inverse process, i.e., -spin-to-charge conversion. Using the PASO quantum material as a fundamental building block, we implement the functionally complete set of logic-in-memory operations and a more complex nonvolatile half-adder logic function. Our work highlights the potential of PASO quantum materials for the development of scalable energy-efficient and ultrafast spintronic computing.
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http://dx.doi.org/10.1126/sciadv.abq6833 | DOI Listing |
Nanoscale Adv
December 2024
The Department of Chemistry & Biochemistry, The University of Texas at El Paso 500 W. University Ave. El Paso TX 79968 USA
Carbon nanomaterials (CNMs), such as carbon nanotubes (CNTs), graphene quantum dots (GQDs), and carbon quantum dots (CQDs), are prevalent in biological systems and have been widely utilized in applications like environmental sensing and biomedical fields. While their presence in human matrices is projected to increase, the interfacial interactions between carbon-based nanoscopic platforms and biomolecular systems continue to remain underexplored. In this study, we investigated the effect of gelatin-sourced CQDs on the globular milk protein beta-lactoglobulin (BLG).
View Article and Find Full Text PDFJ Mater Chem B
January 2025
Department of Chemistry and Biochemistry, The University of Texas at El Paso, 500 West University Avenue, El Paso, Texas 79968, USA.
J Am Chem Soc
December 2024
College of Chemistry, Chemical Engineering and Materials Science, and State Key Laboratory of Radiation Medicine and Protection, Soochow University, Suzhou, Jiangsu 215123, P. R. China.
Water Res
February 2025
Institute of Environmental Research at the Greater Bay Area, Key Laboratory for Water Quality and Conservation of the Pearl River Delta, Ministry of Education, Guangzhou University, Guangzhou 510006, PR China.
Dissolved organic matter (DOM) originating from microplastics (MPs-DOM) is increasingly recognized as a substantial component of aquatic DOM. The photochemistry of MPs-DOM, essential for understanding its environmental fate and impacts, remains largely unexplored. This study investigates the photochemical behaviors of MPs-DOM derived from two common plastics: polystyrene (PS) and polyvinyl chloride (PVC), which represent aromatic and aliphatic plastics, respectively.
View Article and Find Full Text PDFJ Chem Phys
October 2024
Physical Sciences Division, Pacific Northwest National Laboratory, Richland, Washington 99354, USA.
The transformative impact of modern computational paradigms and technologies, such as high-performance computing (HPC), quantum computing, and cloud computing, has opened up profound new opportunities for scientific simulations. Scalable computational chemistry is one beneficiary of this technological progress. The main focus of this paper is on the performance of various quantum chemical formulations, ranging from low-order methods to high-accuracy approaches, implemented in different computational chemistry packages and libraries, such as NWChem, NWChemEx, Scalable Predictive Methods for Excitations and Correlated Phenomena, ExaChem, and Fermi-Löwdin orbital self-interaction correction on Azure Quantum Elements, Microsoft's cloud services platform for scientific discovery.
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