Large-scale kinetic roughening behavior of coffee-ring fronts.

Phys Rev E

Departamento de Física, Universidad de Extremadura, 06006 Badajoz, Spain.

Published: October 2022

We have studied the kinetic roughening behavior of the fronts of coffee-ring aggregates via extensive numerical simulations of the off-lattice model considered for this context [Dias et al., Soft Matter 14, 1903 (2018)1744-683X10.1039/C7SM02136D]. This model describes ballistic aggregation of patchy colloids and depends on a parameter r_{AB} which controls the affinity of the two patches, A and B. Suitable boundary conditions allow us to elucidate a discontinuous pinning-depinning transition at r_{AB}=0, with the front displaying intrinsic anomalous scaling, but with unusual exponent values α≃1.2, α_{loc}≃0.5, β≃1, and z≃1.2. For 00.01 and the system suffers a strong crossover dominated by the r_{AB}=0 behavior for r_{AB}≤0.01. A detailed analysis of correlation functions shows that the aggregate fronts are always in the moving phase for 0

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http://dx.doi.org/10.1103/PhysRevE.106.044801DOI Listing

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