The optical responses of metals are often dominated by plasmonic resonances, that is, the collective oscillations of interacting electron liquids. Here we unveil a new class of plasmons─quantum metric plasmons (QMPs)─that arise in a wide range of parity-violating magnetic metals. In these materials, a dipolar distribution of the quantum metric (a fundamental characteristic of Bloch wave functions) produces intrinsic nonreciprocal bulk plasmons. Strikingly, QMP nonreciprocity manifests even when the single-particle dispersion is symmetric: QMPs are sensitive to time-reversal and parity violations hidden in the Bloch wave function. In materials with asymmetric single-particle dispersions, quantum metric dipole induced nonreciprocity can continue to dominate at large frequencies. We anticipate that QMPs can be realized in a wide range of parity-violating magnets, including twisted bilayer graphene heterostructures, where quantum geometric quantities can achieve large values.
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http://dx.doi.org/10.1021/acs.nanolett.2c03126 | DOI Listing |
J Phys Condens Matter
June 2024
Department of Physics, Graduate School of Science, Kyoto University, Kyoto 606-8502, Japan.
Parity-time-reversal symmetry (PTsymmetry), a symmetry for the combined operations of space inversion (P) and time reversal (T), is a fundamental concept of physics and characterizes the functionality of materials as well asPandTsymmetries. In particular, thePT-symmetric systems can be found in the centrosymmetric crystals undergoing the parity-violating magnetic order which we call the odd-parity magnetic multipole order. While this spontaneous order leavesPTsymmetry intact, the simultaneous violation ofPandTsymmetries gives rise to various emergent responses that are qualitatively different from those allowed by the nonmagneticP-symmetry breaking or by the ferromagnetic order.
View Article and Find Full Text PDFOrig Life Evol Biosph
June 2023
Department of Physics, Alabama A&M University, Huntsville, AL, 35762, USA.
While there is consensus that Archean atmosphere was anoxic with O pressure, p(O) <10 PAL (present atmospheric level) at sea-level, evidence suggests that p(O) at stratospheric altitudes of 10-50 km was orders of magnitude higher, a result of photodissociation of CO by UVC sunlight and incomplete mixing of O with other gases. Molecular O is paramagnetic due to triplet ground state. Magnetic circular dichroism (MCD) by stratospheric O is examined in earth's magnetic field and shows maximum circular polarization │(I - I)│ at altitude of 15-30 km (I/I is intensity of left/right circularly polarized light).
View Article and Find Full Text PDFJ Chem Phys
March 2023
Instituto de Modelado e Innovación Tecnológica, CONICET, and Departamento de Física, Facultad de Ciencias Exactas y Naturales, UNNE, Avenida Libertad 5460, W3404AAS Corrientes, Argentina.
The nuclear-spin-dependent parity-violation contributions to the nuclear magnetic resonance shielding and nuclear spin-rotation tensors (σ and M, respectively) are known to be formally related to one another in the non-relativistic regime. In this work, the polarization propagator formalism and the linear response within the elimination of small components model are used to show a new and more general relationship between them, which is valid within the relativistic framework. The full set of the zeroth- and first-order relativistic contributions to σ and M are also given here for the first time, and these results are compared with previous findings.
View Article and Find Full Text PDFNano Lett
December 2022
Division of Physics and Applied Physics, School of Physical and Mathematical Sciences, Nanyang Technological University, Singapore637371.
The optical responses of metals are often dominated by plasmonic resonances, that is, the collective oscillations of interacting electron liquids. Here we unveil a new class of plasmons─quantum metric plasmons (QMPs)─that arise in a wide range of parity-violating magnetic metals. In these materials, a dipolar distribution of the quantum metric (a fundamental characteristic of Bloch wave functions) produces intrinsic nonreciprocal bulk plasmons.
View Article and Find Full Text PDFThe chiral magnetic effect (CME) refers to charge separation along a strong magnetic field due to imbalanced chirality of quarks in local parity and charge-parity violating domains in quantum chromodynamics. The experimental measurement of the charge separation is made difficult by the presence of a major background from elliptic azimuthal anisotropy. This background and the CME signal have different sensitivities to the spectator and participant planes, and could thus be determined by measurements with respect to these planes.
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