We investigate the effect of manipulating the laser quality factor and the spectral properties of the gain medium on an oligomer-based plasmonic nanolaser. We develop different designs of the oligomer resonators, decreasing the lasing threshold and increasing the mode lifetime to improve the lasing efficiency. Based on the designs we are able to decrease the lasing threshold by a factor of ten. We discuss and show numerically the influence of the oligomer geometry, the lasing mode oscillation lifetime, and the photoluminescence peak linewidth of the gain medium on the lasing efficiency of the oligomer based plasmonic nanolaser.
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http://dx.doi.org/10.1364/OE.472812 | DOI Listing |
Nanoscale
January 2025
Key Laboratory of 3D Micro/Nano Fabrication and Characterization of Zhejiang Province, School of Engineering, Westlake University, 18 Shilongshan Road, Hangzhou 310024, Zhejiang Province, China.
Lowering the population inversion threshold is key to leveraging quantum dots (QDs) for nanoscale lasing and laser miniaturization. However, optical realization of population inversion in QDs has an inherent limitation: the number of excited electrons per QD is bound by the absorbed photons. Here we show that one can break this population limit and realize near-zero threshold inversion plasmonic doping.
View Article and Find Full Text PDFNat Nanotechnol
January 2025
Wellman Center for Photomedicine, Massachusetts General Hospital, Cambridge, MA, USA.
The ultimate limit for laser miniaturization would be achieving lasing action in the lowest-order cavity mode within a device volume of ≤(λ/2n), where λ is the free-space wavelength and n is the refractive index. Here we highlight the equivalence of localized surface plasmons and surface plasmon polaritons within resonant systems, introducing nanolasers that oscillate in the lowest-order localized surface plasmon or, equivalently, half-cycle surface plasmon polariton. These diffraction-limited single-mode emitters, ranging in size from 170 to 280 nm, harness strong coupling between gold and InGaAsP in the near-infrared (λ = 1,000-1,460 nm), away from the surface plasmon frequency.
View Article and Find Full Text PDFNanophotonics
July 2024
School of Physics, The University of Sydney, Sydney, Australia.
As the demand for smaller and more compact lasers increases, the physical dimensions of laser diodes are already at the diffraction limit, which impairs this miniaturization trend and limits direct laser integration into photonic and especially nanophotonic circuits. However, plasmonics has allowed the development of a novel class of lasers that can be manufactured without being limited by diffraction, exhibiting ultralow energy consumption, small volumes, and high modulation speeds that could someday compete with their modern macroscale counterparts. Nevertheless, a wide variety of issues create roadblocks for further development and commercial adoption.
View Article and Find Full Text PDFNanophotonics
March 2024
Laboratory of Integrated Opto-Mechanics and Electronics, School of Optical-Electrical and Computer Engineering, University of Shanghai for Science and Technology, Shanghai 200093, China.
Small
January 2025
College of Chemistry and Chemical Engineering, Lanzhou University, Lanzhou, 730000, China.
Plasmonic nanolasers, which are promising coherent light sources for integrated photonics, super-resolution imaging, and ultrasensitive sensing applications, face the challenge of high thresholds due to inherent losses in plasmonic nanocavities. While considerable efforts have been made to improve the Q factor, typically quantified by the full width at half maximum (FWHM), intensity (ΔI) is another critical feature of plasmonic resonance. However, the combined influence of both the Q factor and resonance intensity of a plasmonic nanocavity on nanolasing threshold has not been sufficiently explored, as experimentally controlling one variable while keeping the other constant is challenging.
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