Farmland nutrient pollution and its evolutionary relationship with plantation economic development in China.

Contradiction between growing plantation economic demand and agro-ecological degradation has always restricted sustainable development of agricultural countries. This study applied the unit inventory analysis to evaluate the productions and discharges of farmland non-point source (FNPS) nitrogen (TN) and phosphorus (TP) among China's nine national-level agricultural districts over 1999-2019. On this basis, we quantified the evolutionary relationship between plantation economic output and FNPS pollution based on optimal regression fitting. The results showed that over 1999-2019, farmland cumulative TN and TP discharges for the whole China were approximately 15807 × 10 t and 1312 × 10 t, with prominent district heterogeneity. According to FNPS discharge magnitudes, China's agricultural districts can be classified into three categories: high, moderate and slight discharge zones. Huang-Huai-Hai Plain and Middle-lower Yangtze Plain were identified as the main severely-polluted districts. Mineral fertilizer is the primary contributor to FNPS pollution. Annual FNPS load showed a trend of increasing followed by decreasing, and the peak interval was recorded in 2014-2016. Spatiotemporal dynamics in FNPS discharge intensities were disparate from that in discharge magnitudes. SC has the highest TN discharge intensity, with an annual average intensity of 0.068 t/ha, followed by MLYP (0.044 t/ha) and HHHP (0.041 t/ha). HHHP has the highest TP discharge intensity, with an annual average intensity of 0.0051 t/ha, followed by SC (0.0038 t/ha) and MLYP (0.0031 t/ha). District-based agro-ecological restoration strategies were accordingly proposed considering FNPS discharge magnitude and intensity concurrently. In most agricultural districts, with the growing economic output in plantation, the FNPS load showed an increase followed by a decrease or to leveling off. Furthermore, with the increasing TN/TP economic partial productivity, the FNPS TN/TP discharge intensities reached the climax, then declined or tended to be flattening out.