High-temperature magnetic skyrmions in BiCrX (X = Se and Te) monolayers.

Phys Chem Chem Phys

College of Physics and Optoelectronic Technology, Collaborative Innovation Center of Rare-Earth Functional Materials and Devices Development, Baoji University of Arts and Sciences, Baoji, 721016, China.

Published: November 2022

Two-dimensional magnetic van der Waals materials provide a fertile platform for the design and control of topological spin textures such as skyrmions. However, despite studies reporting skyrmions in many 2D magnetic systems, those of the hosting van der Waals materials remain limited. Here, first-principles calculations and Monte Carlo simulations, we propose BiCrX as a new family of materials for hosting skyrmions. Due to the large SOC of the X atom and intrinsic inversion asymmetry, an inherent large DMI occurs in all systems, enabling intriguing Néel-type skyrmions. Furthermore, upon applying a moderate magnetic field, isolated skyrmions and skyrmion lattices emerge in our systems, and are robust within a relatively wide temperature range.

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http://dx.doi.org/10.1039/d2cp03476jDOI Listing

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