A multifunctional design based on vanadium dioxide (VO) metamaterial structure is proposed. Broadband absorption, linear-to-linear (LTL) polarization conversion, linear-to-circular (LTC) polarization conversion, and total reflection can be achieved based on the insulator-to-metal transition (IMT) of VO. When the VO is in the metallic state, the multifunctional structure can be used as a broadband absorber. The results show that the absorption rate exceeds 90% in the frequency band of 2.17 - 4.94 THz, and the bandwidth ratio is 77.8%. When VO is in the insulator state, for the incident terahertz waves with a polarization angle of 45°, the structure works as a polarization converter. In this case, LTC polarization conversion can be obtained in the frequency band of 0.1 - 3.5 THz, and LTL polarization conversion also can be obtained in the frequency band of 3.5 - 6 THz, especially in the 3.755 - 4.856 THz band that the polarization conversion rate is over 90%. For the incident terahertz waves with a polarization angle of 0°, the metamaterial structure can be used as a total reflector. Additionally, impacts of geometrical parameters, incidence angle and polarization angle on the operating characteristics have also been investigated. The designed switchable multifunctional metasurfaces are promising for a wide range of applications in advanced terahertz research and smart applications.
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Adv Mater
January 2025
College of Environment and Climate, Guangdong Provincial Key Laboratory of Environmental Pollution and Health, Jinan University, Guangzhou, 510632, China.
Combining piezocatalysts with mechanical ball milling for dissociating water to generate hydroxyl radicals (·OH) offers unprecedented opportunities for energy conversion and environmental remediation. However, the in-depth insights into the relationship between water and local polarization piezoelectric electric field (LPPEF) are currently lacking, in particularly, the ·OH formation mechanism in ball milling driven piezocatalyst system is not systematically elucidated. To this end, the present work constructs a ball milling driven piezoelectric solid/liquid interface between piezoelectric PbBOCl (PBOC) and different contents of water to investigate LPPEF initiated catalytic reaction.
View Article and Find Full Text PDFSci Adv
January 2025
National Laboratory of Solid State Microstructures and School of Physics, Nanjing University, Nanjing 210093, China.
Entangled photon-pair sources are pivotal in various quantum applications. Miniaturizing the quantum devices to meet the requirement in limited space applications drives the search for ultracompact entangled photon-pair sources. The rise of two-dimensional (2D) semiconductors has been demonstrated as ultracompact entangled photon-pair sources.
View Article and Find Full Text PDFNanophotonics
January 2025
Key Laboratory for Information Science of Electromagnetic Waves, School of Information Science and Technology, Fudan University, Shanghai 200433, China.
Gesture recognition plays a significant role in human-machine interaction (HMI) system. This paper proposes a gesture-controlled reconfigurable metasurface system based on surface electromyography (sEMG) for real-time beam deflection and polarization conversion. By recognizing the sEMG signals of user gestures through a pre-trained convolutional neural network (CNN) model, the system dynamically modulates the metasurface, enabling precise control of the deflection direction and polarization state of electromagnetic waves.
View Article and Find Full Text PDFNat Commun
January 2025
Institute of Biomedical Engineering, College of Life Sciences, Qingdao University, Qingdao, China.
The development of acid-stable water oxidation electrocatalysts is crucial for high-performance energy conversion devices. Different from traditional nanostructuring, here we employ an innovative microwave-mediated electron-phonon coupling technique to assemble specific Ru atomic patterns (instead of random Ru-particle depositions) on MnCrO surfaces (Ru-MnCrO) in RuCl solution because hydrated Ru-ion complexes can be uniformly activated to replace some Mn sites at nearby Cr-dopants through microwave-triggered energy coherent superposition with molecular rotations and collisions. This selective rearrangement in Ru-MnCrO with particular spin-differentiated polarizations can induce localized spin domain inversion from reversed to parallel direction, which makes Ru-MnCrO demonstrate a high current density of 1.
View Article and Find Full Text PDFSci Rep
January 2025
Key Laboratory of Micro/nano Devices and Systems, Ministry of Education, North University of China, Taiyuan, 030051, China.
As the hyperentanglement of photon systems holds lots of remarkable applications for enhancing channel capacity with less quantum resource, the interconversion of various hyperentangled states warrants in-depth investigation and becomes a vital work for quantum information technologies. Here we realize completely mutual conversions between spatial-polarization hyperentangled Knill-Laflamme-Milburn state and hyperentangled W state for three-photon systems, resorting to hyperparallel quantum control gates and the practical nonlinear interaction of nitrogen-vacancy centers coupled with whispering-gallery-mode microresonators. The hyperparallel quantum gates, i.
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