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The Other Dimension-Tuning Hole Extraction via Nanorod Width. | LitMetric

The Other Dimension-Tuning Hole Extraction via Nanorod Width.

Nanomaterials (Basel)

Schulich Faculty of Chemistry, The Russell Berrie Nanotechnology Institute, The Nancy and Stephen Grand Technion Energy Program, Technion-Israel Institute of Technology, Haifa 32000, Israel.

Published: September 2022

AI Article Synopsis

Article Abstract

Solar-to-hydrogen generation is a promising approach to generate clean and renewable fuel. Nanohybrid structures such as CdSe@CdS-Pt nanorods were found favorable for this task (attaining 100% photon-to-hydrogen production efficiency); yet the rods cannot support overall water splitting. The key limitation seems to be the rate of hole extraction from the semiconductor, jeopardizing both activity and stability. It is suggested that hole extraction might be improved via tuning the rod's dimensions, specifically the width of the CdS shell around the CdSe seed in which the holes reside. In this contribution, we successfully attain atomic-scale control over the width of CdSe@CdS nanorods, which enables us to verify this hypothesis and explore the intricate influence of shell diameter over hole quenching and photocatalytic activity towards H production. A non-monotonic effect of the rod's diameter is revealed, and the underlying mechanism for this observation is discussed, alongside implications towards the future design of nanoscale photocatalysts.

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Source
http://www.ncbi.nlm.nih.gov/pmc/articles/PMC9565346PMC
http://dx.doi.org/10.3390/nano12193343DOI Listing

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