Challenges and opportunities in continuous flow processes for electrochemically mediated carbon capture.

Carbon capture from both stationary emitters and dilute sources is critically needed to mitigate climate change. Carbon dioxide separation methods driven by electrochemical stimuli show promise to sidestep the high-energy penalty and fossil-fuel dependency associated with the conventional pressure and temperature swings. Compared with a batch process, electrochemically mediated carbon capture (EMCC) operating in a continuous flow mode offers greater design flexibility. Therefore, this review introduces key advances in continuous flow EMCC for point source, air, and ocean carbon captures. Notably, the main challenges and future research opportunities for practical implementation of continuous flow EMCC processes are discussed from a multi-scale perspective, from molecules to electrochemical cells and finally to separation systems.