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Morphology Genetic Metal-Organic Frameworks-Based Biocomposites for Efficient Photocatalytic Hydrogen Evolution. | LitMetric

Morphology Genetic Metal-Organic Frameworks-Based Biocomposites for Efficient Photocatalytic Hydrogen Evolution.

Langmuir

State Key Laboratory of Optoelectronic Materials and Technologies, Nanotechnology Research Center, School of Materials Science & Engineering, Sun Yat-sen University, Guangzhou 510275, China.

Published: September 2022

Metal-organic frameworks (MOFs), MIL-125 and UiO-66, were modified on the butterfly wings (BWs) by chemical bonds, and CdS was grown in situ on them through a solvothermal approach. The BWs enable the biocomposites to possess a wider (>600 nm) and stronger light absorption. The in situ growth method can produce highly active and stable biocomposites. These novel morphologic MOF/CdS biocomposites were characterized using scanning electron microscopy, X-ray diffraction, X-ray photoelectron spectroscopy, and so on. The resulting composites were tested for photocatalytic hydrogen production through water splitting with platinum and lactic acid as the co-catalyst and sacrificial agent, respectively. The two samples showed higher activity than bulk CdS, MOFs, or their composites. Therefore, this paper provides an appropriate method to obtain the MOF/CdS biocomposites, and the resulting biocomposites are proved to be efficient catalyst systems for hydrogen evolution from water under visible light with a wider wavelength.

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Source
http://dx.doi.org/10.1021/acs.langmuir.2c01104DOI Listing

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