A hallmark of strongly correlated quantum materials is the rich phase diagram resulting from competing and intertwined phases with nearly degenerate ground-state energies. A well-known example is the copper oxides, in which a charge density wave (CDW) is ordered well above and strongly coupled to the magnetic order to form spin-charge-separated stripes that compete with superconductivity. Recently, such rich phase diagrams have also been shown in correlated topological materials. In 2D kagome lattice metals consisting of corner-sharing triangles, the geometry of the lattice can produce flat bands with localized electrons, non-trivial topology, chiral magnetic order, superconductivity and CDW order. Although CDW has been found in weakly electron-correlated non-magnetic AVSb (A = K, Rb, Cs), it has not yet been observed in correlated magnetic-ordered kagome lattice metals. Here we report the discovery of CDW in the antiferromagnetic (AFM) ordered phase of kagome lattice FeGe (refs. ). The CDW in FeGe occurs at wavevectors identical to that of AVSb (refs. ), enhances the AFM ordered moment and induces an emergent anomalous Hall effect. Our findings suggest that CDW in FeGe arises from the combination of electron-correlations-driven AFM order and van Hove singularities (vHSs)-driven instability possibly associated with a chiral flux phase, in stark contrast to strongly correlated copper oxides and nickelates, in which the CDW precedes or accompanies the magnetic order.

Download full-text PDF

Source
http://dx.doi.org/10.1038/s41586-022-05034-zDOI Listing

Publication Analysis

Top Keywords

kagome lattice
16
magnetic order
12
charge density
8
density wave
8
rich phase
8
copper oxides
8
lattice metals
8
afm ordered
8
cdw fege
8
cdw
7

Similar Publications

Metal-organic frameworks (MOFs) are a fascinating class of structured materials with diverse functionality originating from the distinctive physicochemical properties. This review focuses on the specific chemical design of geometrically frustrated MOFs along with the origin of the intriguing magnetic properties. We have discussed the arrangement of spin centres (metal and ligand) which are responsible for the unusual magnetic phenomena in MOFs.

View Article and Find Full Text PDF

Janus materials, a novel class of materials with two faces of different chemical compositions and electronic polarities, offer significant potential for various applications with catalytic reactions, chemical sensing, and optical or electronic responses. A key aspect for such functionalities is face-dependent electronic bipolarity, which is usually limited by the chemical distinction of terminated surfaces and has not been exploited in the semiconducting regime. Here, it is showed that a Janus and Kagome van der Waals (vdW) material NbTeI has ferroelectric-like coherent stacking of the Janus layers and hosts strong electronic bipolar states in the semiconducting regime.

View Article and Find Full Text PDF

Electrically conductive coordination polymers (ECCPs), particularly those incorporating benzenehexathiol (BHT) ligands, are emerging as a distinctive class of electronic materials with tunable semiconducting and metallic properties. However, the exploration of novel ECCPs with low-symmetry structures and electrical anisotropy remains under development. Here, we report the on-water surface synthesis of a novel ECCP, namely Cu5BHT, which exhibits a low-symmetry structure and unique in-plane electrical anisotropy that differs from the well-known Cu3BHT phase.

View Article and Find Full Text PDF

Atomic Manipulation on 2D Sumanene for Precise Fermi Level Positioning in Ultrafast High-Capacity Alkali Metal Batteries.

Nano Lett

January 2025

State Key Laboratory of Structural Analysis for Industrial Equipment & School of Physics, Dalian University of Technology, Dalian 116024 People's Republic of China.

Article Synopsis
  • A sumanene monolayer with a unique Kagome-like lattice features two flat bands and two Dirac cones, which can be designed using carbon clusters.
  • First-principles simulations show that surface charge doping can effectively adjust the Fermi level between these bands, allowing for the transformation of the semiconducting monolayer into a semimetal using Li/Na/K atoms.
  • This doped sumanene exhibits high theoretical storage capacity, rapid charge capability, and exceptional structural stability, making it an attractive anode material for alkali-metal batteries.
View Article and Find Full Text PDF

Electronic band evolution between Lieb and kagome nanoribbons.

Nanotechnology

January 2025

Departamento de Física, Universidade Federal do Ceará, Campus do Pici, 60455-900 Fortaleza, Ceará, Brazil.

We investigate the electronic properties of nanoribbons made out of monolayer Lieb, transition, and kagome lattices using the tight-binding model with a generic Hamiltonian. It allows us to map the evolutionary stages of the interconvertibility process between Lieb and kagome nanoribbons by means of only one control parameter. Results for the energy spectra, the density of states, and spatial probability density distributions are discussed for nanoribbons with three types of edges: straight, bearded, and asymmetric.

View Article and Find Full Text PDF

Want AI Summaries of new PubMed Abstracts delivered to your In-box?

Enter search terms and have AI summaries delivered each week - change queries or unsubscribe any time!