We study numerically the role of hydrodynamics in the liquid-hexatic transition of active colloids at intermediate activity, where motility induced phase separation (MIPS) does not occur. We show that in the case of active Brownian particles (ABP), the critical density of the transition decreases upon increasing the particle's mass, enhancing ordering, while self-propulsion has the opposite effect in the activity regime considered. Active hydrodynamic particles (AHP), instead, undergo the liquid-hexatic transition at higher values of packing fraction [Formula: see text] than the corresponding ABP, suggesting that hydrodynamics have the net effect of disordering the system. At increasing densities, close to the hexatic-liquid transition, we found in the case of AHP the appearance of self-sustained organized motion with clusters of particles moving coherently.
Download full-text PDF |
Source |
---|---|
http://www.ncbi.nlm.nih.gov/pmc/articles/PMC9470657 | PMC |
http://dx.doi.org/10.1140/epje/s10189-022-00230-1 | DOI Listing |
Phys Rev E
August 2023
CNRS UMR7083, ESPCI Paris, Université PSL, 10 rue Vauquelin, 75005 Paris, France.
We study the liquid-hexatic transition of soft disks with massively parallel simulations and determine the equation of state as a function of system size. For systems with interactions decaying as the inverse mth power of the separation, the liquid-hexatic phase transition is continuous for m=12 and m=8, while it is of first order for m=24. The critical power m for the transition between continuous and first-order behavior is larger than previously reported.
View Article and Find Full Text PDFPhys Rev E
November 2022
IFISC, Instituto de Física Interdisciplinar y Sistemas Complejos (CSIC-UIB), Campus Universitat de les Illes Balears, E-07122 Palma de Mallorca, Spain.
We study the effects of stochastic birth and death processes on the structural phases of systems of active and passive Brownian particles subject to volume exclusion. The total number of particles in the system is a fluctuating quantity, determined by the birth and death parameters and on the activity of the particles. As the birth and death parameters are varied, we find liquid, hexatic, and solid phases.
View Article and Find Full Text PDFEur Phys J E Soft Matter
September 2022
Dipartimento di Fisica, Università degli Studi di Bari and INFN, Sezione di Bari, via Amendola 173, Bari, 70126, Italy.
We study numerically the role of hydrodynamics in the liquid-hexatic transition of active colloids at intermediate activity, where motility induced phase separation (MIPS) does not occur. We show that in the case of active Brownian particles (ABP), the critical density of the transition decreases upon increasing the particle's mass, enhancing ordering, while self-propulsion has the opposite effect in the activity regime considered. Active hydrodynamic particles (AHP), instead, undergo the liquid-hexatic transition at higher values of packing fraction [Formula: see text] than the corresponding ABP, suggesting that hydrodynamics have the net effect of disordering the system.
View Article and Find Full Text PDFJ Chem Phys
September 2019
Energy Institute and Department of Chemical Engineering, City College of New York, New York, New York 10031, USA.
The determination of phase behavior and, in particular, the nature of phase transitions in two-dimensional systems is often clouded by finite size effects and by access to the appropriate thermodynamic regime. We address these issues using an alternative route to deriving the equation of state of a two-dimensional hard-core particle system, based on kinetic arguments and the Gibbs adsorption isotherm, by the use of the random sequential adsorption with a surface diffusion model. Insight into coexistence regions and phase transitions is obtained through direct visualization of the system at any fractional surface coverage via local bond orientation order.
View Article and Find Full Text PDFNat Commun
November 2018
Laboratoire de Physique Statistique, Département de physique de l'ENS, Ecole Normale Supérieure, PSL Research University, Université Paris Diderot, Sorbonne Paris Cité, Sorbonne Universités, UPMC Univ. Paris 06, CNRS, 75005, Paris, France.
Active matter has been much studied for its intriguing properties such as collective motion, motility-induced phase separation and giant fluctuations. However, it has remained unclear how the states of active materials connect with the equilibrium phases. For two-dimensional systems, this is also because the understanding of the liquid, hexatic, and solid equilibrium phases and their phase transitions is recent.
View Article and Find Full Text PDFEnter search terms and have AI summaries delivered each week - change queries or unsubscribe any time!