The near-surface temperature prediction (NTP) is an important spatial-temporal forecast problem, which can be used to prevent temperature crises. Most of the previous approaches fail to explicitly model the long- and short-range spatial correlations simultaneously, which is critical to making an accurate temperature prediction. In this study, both long- and short-range spatial correlations are captured to fill this gap by a novel convolution operator named Long- and Short-range Convolution (LS-Conv). The proposed LS-Conv operator includes three key components, namely, Node-based Spatial Attention (NSA), Long-range Adaptive Graph Constructor (LAGC), and Long- and Short-range Integrator (LSI). To capture long-range spatial correlations, NSA and LAGC are proposed to evaluate node importance aiming at auto-constructing long-range spatial correlations, which is named as Long-range aware Graph Convolution Network (LR-GCN). After that, the Short-range aware Convolution Neural Network (SR-CNN) accounts for the short-range spatial correlations. Finally, LSI is proposed to capture both long- and short-range spatial correlations by intra-unifying LR-GCN and SR-CNN. Upon the proposed LS-Conv operator, a new model called Long- and Short-range for NPT (LS-NTP) is developed. Extensive experiments are conducted on two real-world datasets and the results demonstrate that the proposed method outperforms state-of-the-art techniques. The source code is available on GitHub:https://github.com/xuguangning1218/LS_NTP.
Download full-text PDF |
Source |
---|---|
http://dx.doi.org/10.1016/j.neunet.2022.07.022 | DOI Listing |
Inorg Chem
December 2024
School of Chemistry and Biochemistry, Georgia Institute of Technology, Atlanta, Georgia 30332, United States.
The interplay between quantum effects from magnetic frustration, low-dimensionality, spin-orbit coupling, and crystal electric field in rare-earth materials leads to nontrivial ground states with unusual magnetic excitations. Here, we investigate YbTaO, which hosts a buckled square net of Yb ions with = 1/2 moments. The observed Curie-Weiss temperature is about -1 K, implying an antiferromagnetic coupling between the Yb moments.
View Article and Find Full Text PDFFront Chem
December 2024
Department of Physics, North Dakota State University, Fargo, ND, United States.
Lattice-based mean-field models of ionic liquids neglect charge discreteness and ion correlations. To address these limitations, we propose separating the short-range and long-range parts of the electrostatic interaction by truncating the Coulomb potential below a fixed distance that is equal to or slightly larger than that between neighboring ions. Interactions and correlations between adjacent ions can then be modeled explicitly, whereas longer-ranged electrostatic interactions are captured on the mean-field level.
View Article and Find Full Text PDFJ Chem Phys
December 2024
Department of Chemistry, Sikkim University, Gangtok 737102, India.
Crystallization and amorphization are important processes and different cooling rates cause these transitions. Obtaining pure metals from their molten state is a challenge unless these two are well understood. Here we study both these transitions in liquid Ti using molecular dynamics simulations wherein Ti is modeled with embedded atom potential.
View Article and Find Full Text PDFJ Phys Chem Lett
December 2024
Institute for Theoretical Physics, TU Wien, Wiedner Hauptstraße 8-10/136, A-1040 Vienna, Austria.
Many-electron correlation methods offer a systematic approach to predicting material properties with high precision. However, practically attaining accurate ground-state properties for bulk metals presents significant challenges. In this work, we propose a novel scheme to reach the thermodynamic limit of the total ground-state energy of metals using coupled cluster theory.
View Article and Find Full Text PDFACS Appl Mater Interfaces
December 2024
Department of Chemistry, Material Science Lab, Annamalai University, Annamalai Nagar, Tamilnadu 608 002, India.
Herein, we demonstrated that a polycrystalline cobalt oxide/borate (CoO-Bo) hybrid catalyst prepared by coprecipitation followed a simple annealing process with a viable boron source of less hazardous ammonium borate, an efficient electrocatalyst for the oxygen evolution reaction (OER). The borate species in the crystalline cobalt oxide lattice provides a tunable polycrystalline morphology with a defect-rich lattice and numerous grain boundaries in the CoO-Bo hybrid electrocatalyst, which significantly boosts the OER activity compared to the crystalline counterparts of CoO and precious IrO in a harsh alkaline electrolyte (1 M KOH). The borate modulated CoO-Bo achieves a 10 mA/cm geometrical current density for the OER with a very low overpotential (η) of 271 mV and small Tafel slope of 34 mV dec, in an inert glassy carbon (GC) support, while only requiring η of 267 and 32 mV dec in a 3D nickel foam (NF) support at the same current density.
View Article and Find Full Text PDFEnter search terms and have AI summaries delivered each week - change queries or unsubscribe any time!