The dilemma of diminishing freshwater resources caused by water pollution has always impacted human life. Solar-driven interfacial evaporation technology has the potential for freshwater production via solar-driven distillation. However, in solar-driven interfacial evaporation technology, it is difficult to overcome the problem of wastewater containing various contaminants. In this work, we propose a bifunctional fabric created by depositing titanium dioxide@carbon black nanoparticles onto cotton fabric (TiO@CB/CF). The TiO@CB/CF has a coupling effect that includes the photothermal effect of CB and photocatalysis of TiO, and it can not only generate clean water but can also purify contaminated water. The resulting bifunctional fabric can achieve an outstanding water evaporation rate of 1.42 kg m h and a conversion efficiency of 90.4% in methylene blue (MB) solution under one-sun irradiation. Simultaneously, the TiO@CB/CF demonstrates a high photocatalytic degradation of 57% for MB solution after 2 h with light irradiation. It still shows a good photocatalysis effect, even when reused in an MB solution for eight cycles. Furthermore, the TiO@CB/CF delivers excellent performance for actual industrial textile dyeing wastewater. This bifunctional fabric has a good application prospect and will provide a novel way to resolve the issue of freshwater scarcity.
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http://dx.doi.org/10.3390/ma15175917 | DOI Listing |
Sci Rep
January 2025
FEMTO-ST Institute (UMR CNRS 6174), UBFC/UTBM. Site de Montbéliard, 90010, Belfort, France.
Seawater electrolysis is an ideal technology for obtaining clean energy-green hydrogen. Developing efficient bifunctional catalysts is crucial for hydrogen production through direct seawater electrolysis. Currently, metal substrates loaded with active catalysts are widely employed as electrodes for seawater electrolysis.
View Article and Find Full Text PDFChem Asian J
January 2025
Birla Institute of Technology and Science, Vidya Vihar, 333031, Pilani, INDIA.
Development of a competent and stable electrocatalyst coupled with photovoltaic system for the generation of green hydrogen, can be a plausible answer to the existing energy crisis. Herein, we have developed Ru doped Ni0.95Se via hydrothermal method as a bifunctional catalyst for overall water splitting coupled with photovoltaic system.
View Article and Find Full Text PDFJ Colloid Interface Sci
January 2025
State Key Laboratory of Chem/Bio-Sensing and Chemometrics, Advanced Catalytic Engineering Research Center of the Ministry of Education, College of Chemistry and Chemical Engineering, Hunan University, Changsha 410082 PR China. Electronic address:
High-entropy phosphides (HEPs) have garnered increasing interest as innovative electrocatalysts for water splitting, highlighted by their distinctive catalytic activity, elemental synergy, and tunable electronic configuration. Herein, a novel electrode comprising CoNiCuZnFeP nanocubes with rich phosphorus vacancies was fabricated through coprecipitation and phosphorization two-step method. The synergistic interaction among metal elements and the modulation of the electronic configuration by phosphorus vacancies augmentation enhance the catalytic performance for both the oxygen evolution reaction (OER) and hydrogen evolution reaction (HER).
View Article and Find Full Text PDFJ Colloid Interface Sci
January 2025
Alan G. MacDiarmid Institute, College of Chemistry, Jilin University, 2699 Qianjin Street, Changchun 130012, PR China. Electronic address:
Water electrolysis represents a green and efficient strategy for hydrogen (H) production. However, the four-electron transfer process involved in its anodic oxygen evolution reaction (OER) half-reaction restricts the H generation rate. Employing hydrazine oxidation reaction (HzOR) as a substitute for OER in H generation can dramatically reduce energy consumption.
View Article and Find Full Text PDFAngew Chem Int Ed Engl
January 2025
Fujian University of Technology, College of Ecological Environment and Urban Construction, 69, Xuefu South Road, Fuzhou 350118, China, 350118, Fuzhou, CHINA.
Rational exploration of cost-effective, durable, and high-performance electrode materials is imperative for advancing the progress of capacitive deionization (CDI). The integration of multicomponent layered double hydroxides (LDHs) with conjugated conductive metal-organic frameworks (c-MOFs) to fabricate bifunctional heterostructure electrode materials is considered a promising strategy. Herein, the fabrication of hierarchical conductive MOF/LDH/CF nanoarchitectures (M-CAT/LDH/CF) as CDI anodes via a controllable grafted-growth strategy is reported.
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