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Hydrophobic Biodegradable Hyperbranched Copolymers with Excellent Marine Diatom Resistance. | LitMetric

Hydrophobic Biodegradable Hyperbranched Copolymers with Excellent Marine Diatom Resistance.

Biomacromolecules

State Key Laboratory of Pollution Control and Resources Reuse, School of the Environment, Nanjing University, Nanjing 210023, China.

Published: October 2022

AI Article Synopsis

Article Abstract

As the utilization of degradable polymer coatings increased, the accompanying trade-off between good degradability and high-efficiency antidiatom adhesion due to their hydrophobic nature remains unresolved. The study presents a new hydrophobic surface-fragmenting coating consisting of degradable hyperbranched polymers (hereafter denoted as h-LLA) synthesized by reversible complexation-mediated copolymerization with isobornyl acrylate (IBOA) and divinyl-functional oligomeric poly(l-lactide) (OLLA-V), both derived from biomass, that exhibited superior resistance (∼0 cell mm) to marine diatom () attachment with higher OLLA content. The combined impact of the microscale hollow semisphere micelles that self-assembled degradable hyperbranched copolymers and hydrolysis-driven self-renewable surfaces following immersion in seawater may account for the remarkable resistance of h-LLA coatings against . Detailed investigations were conducted across multiple perspectives, from hydrolytic degradation to broad-spectrum antibacterial attachment to ecotoxicity assessment. The excellent features of high resistance to marine diatoms and bacterial attachment, degradability, and environmental friendliness make the as-prepared h-LLA coatings widely sought after for antifouling coating applications.

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Source
http://dx.doi.org/10.1021/acs.biomac.2c00779DOI Listing

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