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Efficient covalent capping of carbon and gold with TEMPO for catalysis and spin writing. | LitMetric
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Efficient covalent capping of carbon and gold with TEMPO for catalysis and spin writing.

Vitalijs Romanovs Valery Sidorkin Evgeniya Doronina Viatcheslav Jouikov

Chem Commun (Camb)

UMR 6226 ISCR, University of Rennes 1, 35042 Rennes, France.

Published: September 2022

Covalent immobilization of TEMPO at carbon and gold an aliphatic -(CH)- linker was achieved cathodic grafting of a diamagnetic precursor, tetramethylpiperidine, with subsequent >NH to >NO oxidation to give TEMPO-capped paramagnetic interfaces ( = 5.2 × 10 mol cm); catalytic and spin switching potential of the thus prepared systems was demonstrated.

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 Source
http://dx.doi.org/10.1039/d2cc01520jDOI Listing

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