We present a theory on the quantum phase diagram of AB-stacked MoTe_{2}/WSe_{2} using a self-consistent Hartree-Fock calculation performed in the plane-wave basis, motivated by the observation of topological states in this system. At filling factor ν=2 (two holes per moiré unit cell), Coulomb interaction can stabilize a Z_{2} topological insulator by opening a charge gap. At ν=1, the interaction induces three classes of competing states, spin density wave states, an in-plane ferromagnetic state, and a valley polarized state, which undergo first-order phase transitions tuned by an out-of-plane displacement field. The valley polarized state becomes a Chern insulator for certain displacement fields. Moreover, we predict a topological charge density wave forming a honeycomb lattice with ferromagnetism at ν=2/3. Future directions on this versatile system hosting a rich set of quantum phases are discussed.
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http://dx.doi.org/10.1103/PhysRevLett.129.056804 | DOI Listing |
Nat Nanotechnol
January 2024
School of Applied and Engineering Physics, Cornell University, Ithaca, NY, USA.
Sci Adv
March 2023
Center for Computational Quantum Physics, Flatiron Institute, New York, NY 10010, USA.
We theoretically study the interplay between magnetism and a heavy Fermi liquid in the AB-stacked transition metal dichalcogenide bilayer system, MoTe/WSe, in the regime in which the layer supports localized magnetic moments coupled by interlayer electron tunneling to a weakly correlated band of itinerant electrons in the layer. We show that the interlayer electron transfer leads to a chiral Kondo exchange, with consequences including a strong dependence of the Kondo temperature on carrier concentration and anomalous Hall effect due to a topological hybridization gap. The theoretical model exhibits two phases, a small Fermi surface magnet and a large Fermi surface heavy Fermi liquid; at the mean-field level, the transition between them is first order.
View Article and Find Full Text PDFNature
April 2023
Kavli Institute at Cornell for Nanoscale Science, Cornell University, Ithaca, NY, USA.
The Kondo lattice-a matrix of local magnetic moments coupled through spin-exchange interactions to itinerant conduction electrons-is a prototype of strongly correlated quantum matter. Usually, Kondo lattices are realized in intermetallic compounds containing lanthanide or actinide. The complex electronic structure and limited tunability of both the electron density and exchange interactions in these bulk materials pose considerable challenges to studying Kondo lattice physics.
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