We present a reanalysis (using the Minnaert limb-darkening approximation) of visible/near-infrared (0.3-2.5 μm) observations of Uranus and Neptune made by several instruments. We find a common model of the vertical aerosol distribution i.e., consistent with the observed reflectivity spectra of both planets, consisting of: (a) a deep aerosol layer with a base pressure >5-7 bar, assumed to be composed of a mixture of HS ice and photochemical haze; (b) a layer of photochemical haze/ice, coincident with a layer of high static stability at the methane condensation level at 1-2 bar; and (c) an extended layer of photochemical haze, likely mostly of the same composition as the 1-2-bar layer, extending from this level up through to the stratosphere, where the photochemical haze particles are thought to be produced. For Neptune, we find that we also need to add a thin layer of micron-sized methane ice particles at ∼0.2 bar to explain the enhanced reflection at longer methane-absorbing wavelengths. We suggest that methane condensing onto the haze particles at the base of the 1-2-bar aerosol layer forms ice/haze particles that grow very quickly to large size and immediately "snow out" (as predicted by Carlson et al. (1988), https://doi.org/10.1175/1520-0469(1988)045<2066:CMOTGP>2.0.CO;2), re-evaporating at deeper levels to release their core haze particles to act as condensation nuclei for HS ice formation. In addition, we find that the spectral characteristics of "dark spots", such as the Voyager-2/ISS Great Dark Spot and the HST/WFC3 NDS-2018, are well modelled by a darkening or possibly clearing of the deep aerosol layer only.
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http://dx.doi.org/10.1029/2022JE007189 | DOI Listing |
Environ Sci Technol
January 2025
Key Laboratory for Semi-Arid Climate Change of the Ministry of Education, College of Atmospheric Sciences, Lanzhou University, Lanzhou 730000, China.
The record-breaking 2019-2020 Australian wildfires have been primarily linked to climate change and its internal variability. However, the meteorological feedback mechanisms affecting smoke dispersion and wildfire emissions on a synoptic scale remain unclear. This study focused on the largest wildfires occurring between December 25, 2019 and January 10, 2020, under the enhanced subtropical high, when the double peak in wildfire evolution was favored by sustained low humidity and two synchronous increases in temperature and wind.
View Article and Find Full Text PDFEnviron Pollut
December 2024
State Key Laboratory of Atmospheric Boundary Layer Physics and Atmospheric Chemistry, Institute of Atmospheric Physics, Chinese Academy of Sciences, Beijing, 100029, China; College of Earth and Planetary Sciences, University of Chinese Academy of Sciences, Beijing, 100049, China.
A multiple-site filter-sampling observation study was conducted in a coastal industrial city (Rizhao, 35°10'59″N, 119°23'57″E) to understand the main components, formation mechanisms, and potential sources of particulate matter. The average (±σ) mass concentration of PM across all the sites was 42 (±27) μg/m, with high variability (6-202 μg/m). Water-soluble inorganic ions (WSIIs) were the major contributors (54%-60%) to PM with mean values for sulfate (13 μg/m), nitrate (6 μg/m), and ammonium (7 μg/m) (SNA).
View Article and Find Full Text PDFEnviron Sci Pollut Res Int
December 2024
Department of Physics, DDU Gorakhpur University, Gorakhpur, 273009, India.
The pristine Himalayas are sensitive to pollutants from different source regions, including its foothills that have adverse effects on air quality and climate. Despite this, there are no observations of aromatic hydrocarbons in the central Himalayas. Thus, online observations of aromatics (C-C, defined here as BTEX) were conducted for the first time at the mountain site (Nainital, 1958 m) in the central Himalayas during January 2017-December 2022 period.
View Article and Find Full Text PDFACS ES T Eng
January 2024
Department of Chemical and Environmental Engineering, University of Cincinnati, Cincinnati, Ohio 45221, United States.
The COVID-19 pandemic has resulted in significant changes in our daily lives, including the widespread use of face masks. Face masks have been reported to reduce the transmission of viral infections by droplets; however, improper use and/or treatment of these masks can cause them to be contaminated, thereby reducing their efficacy. Moreover, regular replacement of face masks is essential to maintaining their effectiveness, which can be challenging in resource-limited healthcare settings.
View Article and Find Full Text PDFACS Earth Space Chem
December 2024
Department of Chemistry, University of Colorado Boulder Boulder, Colorado 80309, United States.
Iodine in the atmosphere destroys ozone and can nucleate particles by formation of iodic acid, HIO. Recent field observations suggest iodate recycles from particles sustaining significant gas-phase IO radical concentrations (0.06 pptv) in aged stratospheric air, and in elevated dust plumes.
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