Local Plastic Response and Slow Heterogeneous Dynamics of Supercooled Liquids.

Phys Rev Lett

Division of Physics and Applied Physics, School of Physical and Mathematical Sciences, Nanyang Technological University, Singapore 637371, Singapore, CNR-SPIN, Dipartimento di Scienze Fisiche, Università di Napoli Federico II, I-80126, Napoli, Italy and CNRS@CREATE LTD, 1 Create Way, No. 08-01 CREATE Tower, Singapore 138602, Singapore.

Published: June 2022

We demonstrate, via numerical simulations, that the relaxation dynamics of supercooled liquids correlates well with a plastic length scale measuring a particle's response to impulsive localized perturbations and weakly to measures of local elasticity. We find that the particle averaged plastic length scale vanishes linearly in temperature and controls the super-Arrhenius temperature dependence of the relaxation time. Furthermore, we show that the plastic length scale of individual particles correlates with their typical displacement at the relaxation time. In contrast, the local elastic response only correlates with the dynamics on the vibrational timescale.

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http://dx.doi.org/10.1103/PhysRevLett.128.258001DOI Listing

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