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Exploring Biomineralization Processes Using In Situ Liquid Transmission Electron Microscopy: A Review.
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January 2025
Department of Materials Science and Engineering, McMaster University, Hamilton, ON, L8S 4L7, Canada.
Liquid transmission electron microscopy (TEM) is a newly established technique broadly used to study reactions in situ. Since its emergence, complex and multifaceted biomineralization processes have been revealed with real-time resolution, where classical and non-classical mineralization pathways have been dynamically observed primarily for Ca and Fe-based mineral systems in situ. For years, classical crystallization pathways have dominated theories on biomineralization progression despite observations of non-traditional routes involving precursor phases using traditional- and cryo-TEM.
View Article and Find Full Text PDFMulti-particle quantum walks on 3D integrated photonic chip.
Light Sci Appl
October 2024
Center for Integrated Quantum Information Technologies (IQIT), School of Physics and Astronomy and State Key Laboratory of Advanced Optical Communication Systems and Networks, Shanghai Jiao Tong University, Shanghai, 200240, China.
Quantum walks provide a speed-up in computational power for various quantum algorithms and serve as inspiration for the construction of complex graph representations. Many pioneering works have been dedicated to expanding the experimental state space and the complexity of graphs. However, these experiments are mostly limited to small experimental scale, which do not reach a many-body level and fail to reflect the multi-particle quantum interference effects among non-adjacent modes.
View Article and Find Full Text PDFDative Bonding Activation Enables Precise Functionalization of the Remote B-H Bond of -Carborane Clusters.
J Am Chem Soc
September 2024
State Key Laboratory of Coordination Chemistry, Jiangsu Key Laboratory of Advanced Organic Materials, School of Chemistry and Chemical Engineering, Nanjing University, Nanjing 210023, China.
The innovation of synthetic strategies for selective B-H functionalization is a pivotal objective in the realm of boron cluster chemistry. However, the precise, efficient, and rapid functionalization of a B-H bond of carboranes that is distant from the existing functional groups remains intractable owing to the limited approaches for site-selective control from the established methods. Herein, we report a dative bonding activation strategy for the selective functionalization of a nonclassical remote B-H site of -carboranes.
View Article and Find Full Text PDFA microscopic approach to crystallization: Challenging the classical/non-classical dichotomy.
J Chem Phys
September 2024
Center for Nonlinear Phenomena and Complex Systems CP 231, Université Libre de Bruxelles, Blvd. du Triomphe, 1050 Brussels, Belgium.
We present a fundamental framework for the study of crystallization based on a combination of classical density functional theory and fluctuating hydrodynamics that is free of any assumptions regarding order parameters and that requires no input other than molecular interaction potentials. We use it to study the nucleation of both droplets and crystalline solids from a low-concentration solution of colloidal particles using two different interaction potentials. We find that the nucleation pathways of both droplets and crystals are remarkably similar at the early stages of nucleation until they diverge due to a rapid ordering along the solid pathways in line with the paradigm of "non-classical" crystallization.
View Article and Find Full Text PDF4D Biochemical Photocustomization of Hydrogel Scaffolds for Biomimetic Tissue Engineering.
Acc Mater Res
August 2023
Department of Chemical Engineering, University of Washington, Seattle, Washington 98105, United States; Department of Bioengineering, Department of Chemistry, Institute of Stem Cell & Regenerative Medicine, Molecular Engineering & Sciences Institute, and Institute for Protein Design, University of Washington, Seattle, Washington 98105, United States.
Programmable engineered tissues and the materials that support them are instrumental to the development of next-generation therapeutics and gaining new understanding of human biology. Toward these ends, recent years have brought a growing emphasis on the creation of "4D" hydrogel culture platforms-those that can be customized in 3D space and on demand over time. Many of the most powerful 4D-tunable biomaterials are photochemically regulated, affording users unmatched spatiotemporal modulation through high-yielding, synthetically tractable, and cytocompatible reactions.
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