Shale Gas Decarbonization in the Permian Basin: Is It Possible?

The United States is unique in the energy reserves held in shale gas fields, which coproduce natural gas and natural gas liquids. Use of this resource, however, contributes to greenhouse gas emissions and, correspondingly, climate change. We explore how natural gas and natural gas liquids might build bridges toward low-carbon transportation fuels. For example, as petroleum refineries produce less gasoline in response to widespread electrification, natural gas liquids can be converted to fuel. We consider whether the greenhouse gas emissions from production and use of these fuels might be offset through three potential outcomes of converting coproduced natural gas to CO through steam methane reforming. First, the CO could be injected into conventional oil formations for enhanced oil recovery. Second, it could be sequestered into saline aquifers to avoid CO emissions from the produced oil combustion. Third, it could be injected into unconventional gas formations in the form of CO-based fracturing fluids. Simultaneously, the coproduced hydrogen from steam methane reforming could be used to support the expansion of the hydrogen economy. The region of study is the Permian Basin. The results show sizeable emission benefits by decreasing net emissions of natural gas production and use to 28 from 88 g-COe/MJ. For revenue generating pathways, a partial decarbonization of 3.4 TCF/year is possible. All of the natural gas can be partially decarbonized if the CO is sequestered in saline aquifers. Overall, the results show that while greenhouse gas emissions can be reduced through decarbonization approaches relying on subsurface sequestration, full natural gas decarbonization is not achieved but must be pursued through other approaches.