Perturbation theory of scattering for grazing-incidence fast-atom diffraction.

Phys Chem Chem Phys

Chemical and Biological Physics Department, Weizmann Insitute of Science, 76100 Rehovoth, Israel.

Published: July 2022

Recent grazing-incidence, fast atom diffraction (GIFAD) experiments have highlighted the well known observation that the distance between classical rainbow angles depends on the incident energy. The GIFAD experiments imply an incident vertical scattering angle, facilitating an analytic analysis using classical perturbation theory, which leads to the conclusion that the so called "dynamic corrugation" amplitude, as defined by Bocan , , 2020 , 096101 is, within first-order perturbation theory, proportional to the tangent of the rainbow angle. Therefore it provides no further information about the interaction than is gleaned from the rainbow angle and its energy dependence. Perhaps more importantly, the resulting analytic theory reveals how the energy dependence of rainbow angles may be inverted into information on the force field governing the interaction of the incident projectile with the surface.

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Source
http://dx.doi.org/10.1039/d2cp01013eDOI Listing

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