One of the most important devices emerging from quantum technology are quantum batteries. However, self-discharging, the process of charge wasting of quantum batteries due to decoherence phenomenon, limits their performance, measured by the concept of ergotropy and half-life time of the quantum battery. The effects of local field fluctuation, introduced by the disorder term in the Hamiltonian of the system, on the performance of the quantum batteries is investigated in this paper. The results reveal that the disorder term could compensate disruptive effects of the decoherence, i.e., self-discharging, and hence improve the performance of the quantum battery via "incoherent gain of ergotropy" procedure. Adjusting the strength of the disorder parameter to a proper value and choosing a suitable initial state of the quantum battery, the amount of free ergotropy, defined with respect to the free Hamiltonian, could exceed the amount of initial stored ergotropy. In addition harnessing the degree of the disorder parameter could help to enhance the half-life time of the quantum battery. This study opens perspective to further investigation of the performance of quantum batteries that explore disorder and many-body effects.
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http://dx.doi.org/10.1103/PhysRevE.105.054115 | DOI Listing |
Molecules
January 2025
Department of Chemistry, Sapienza University of Rome, P. le Aldo Moro 5, 00185 Rome, Italy.
In this paper, we present a molecular dynamics study of the structural and dynamical properties of γ-valerolactone (GVL) both as a standalone solvent and in electrolyte formulations for electrochemistry applications. This study involves developing a new parameterization of a polarizable forcefield and applying it to simulate pure GVL and selected salt solutions. The forcefield was validated with experimental bulk data and quantum mechanical calculations, with excellent agreement obtained in both cases.
View Article and Find Full Text PDFEntropy (Basel)
January 2025
Department of Physics, MIT, Cambridge, MA 02139, USA.
Maximizing the amount of work harvested from an environment is important for a wide variety of biological and technological processes, from energy-harvesting processes such as photosynthesis to energy storage systems such as fuels and batteries. Here, we consider the maximization of free energy-and by extension, the maximum extractable work-that can be gained by a classical or quantum system that undergoes driving by its environment. We consider how the free energy gain depends on the initial state of the system while also accounting for the cost of preparing the system.
View Article and Find Full Text PDFJ Phys Chem Lett
January 2025
Key Laboratory of Physics and Technology for Advanced Batteries, Ministry of Education, College of Physics, Jilin University, Qianjin Street No. 2699, Changchun 130012, China.
Developing heavy-metal-free materials with wide tunable emission is important to light-emitters. The alloying method is utilized in ZnSe magic size clusters (MSCs) with Te to form ZnSeTe and manipulate the band gap structure in ZnSe. The growth of ZnTe on alloyed ZnSeTe quantum dots (QDs) forms ZnSeTe/ZnTe core/shell nanostructures, showing the tunable photoluminescence emission peak from 450 to 760 nm with the different thicknesses of ZnTe shell.
View Article and Find Full Text PDFNanoscale
January 2025
MOE Key Laboratory of New Processing Technology for Nonferrous Metals and Materials, School of Resources, Environment and Materials, Guangxi University, Nanning 530004, China.
The CO reduction reaction (CORR) and oxygen reduction reaction (ORR) show great promise for expanding the use of renewable energy sources and fostering carbon neutrality. Sn-based catalysts show CORR activity; however, they have been rarely reported in the ORR. Herein, we prepared a nitrogen-carbon structure loaded with Fe-doped Sn nanoparticles (Fe-Sn/NC), which has good ORR and CORR activity.
View Article and Find Full Text PDFSmall
January 2025
MEET, Battery Research Center, University of Muenster, 48149, Muenster, Germany.
Rechargeable lithium-ion batteries (LIBs) are critical for enabling sustainable energy storage. The capacity of cathode materials is a major limiting factor in the LIB performance, and doping has emerged as an effective strategy for enhancing the electrochemical properties of nickel-rich layered oxides such as NCM811. In this study, boron is homogeneously incorporated into the tetrahedral site of NCM811 through co-precipitation, leading to an inductive effect on transition metal (TM)-O-B bonds that delayed structural collapse and reduced oxygen release.
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