Cuprate superconductors have the highest critical temperatures (T) at ambient pressure, yet a consensus on the superconducting mechanism remains to be established. Finding an empirical parameter that limits the highest reachable T can provide crucial insight into this outstanding problem. Here, in the first two Ruddlesden-Popper members of the model Hg-family of cuprates, which are chemically nearly identical and have the highest T among all cuprate families, we use inelastic photon scattering to reveal that the energy of magnetic fluctuations may play such a role. In particular, we observe the single-paramagnon spectra to be nearly identical between the two compounds, apart from an energy scale difference of ~30% which matches their difference in T. The empirical correlation between paramagnon energy and maximal T is further found to extend to other cuprate families with relatively high T's, hinting at a fundamental connection between them.
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http://www.ncbi.nlm.nih.gov/pmc/articles/PMC9174205 | PMC |
http://dx.doi.org/10.1038/s41467-022-30918-z | DOI Listing |
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