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LiNiMnO-Hybridized Gel Polymer Cathode and Gel Polymer Electrolyte Containing a Sulfolane-Based Highly Concentrated Electrolyte for the Fabrication of a 5 V Class of Flexible Lithium Batteries. | LitMetric

AI Article Synopsis

  • * A new hybridized gel polymer cathode and a gel polymer electrolyte, both using a special concentrated electrolyte, were successfully developed, allowing for easy battery assembly without needing to inject the electrolyte.
  • * The battery cells exhibited great capacity retention even when subjected to constant bending or deformation, showcasing a scalable method for making reliable 5 V batteries suitable for flexible applications.

Article Abstract

The design and fabrication of lithium secondary batteries with a high energy density and shape flexibility are essential for flexible and wearable electronics. In this study, we fabricated a high-voltage (5 V class) flexible lithium polymer battery using a lithium nickel manganese oxide (LiNiMnO) cathode. A LiNiMnO-hybridized gel polymer cathode (GPC) and a gel polymer electrolyte (GPE) membrane, both containing a sulfolane (SL)-based highly concentrated electrolyte (HCE), enabled the fabrication of a polymer battery by simple lamination with a metallic lithium anode, where the injection of the electrolyte solution was not required. GPC with high flexibility has a hierarchically continuous three-dimensional porous architecture, which is advantageous for forming continuous ion-conduction paths. The GPE membrane has significant ionic conductivity enough for reliable capacity delivery. Therefore, the fabricated lithium polymer pouch cells demonstrated excellent capacity retention under continuous deformation conditions. This study provides a promising strategy for the fabrication of scalable and flexible 5 V class batteries using GPC and GPE containing SL-based HCE.

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Source
http://www.ncbi.nlm.nih.gov/pmc/articles/PMC9161388PMC
http://dx.doi.org/10.1021/acsomega.2c00861DOI Listing

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