[This corrects the article DOI: 10.1039/D0RA02558E.].
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| http://dx.doi.org/10.1039/d0ra90092c | DOI Listing |
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Correction: Tantalum(v) 1,3-propanediolate β-diketonate solution as a precursor to sol-gel derived, metal oxide thin films.
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August 2020
IBI-3, Bioelectronics, Forschungszentrum Jülich GmbH D-52425 Germany
[This corrects the article DOI: 10.1039/D0RA02558E.].
View Article and Find Full Text PDFDesigning catalysts for nitrene transfer using early transition metals and redox-active ligands.
Inorg Chem
October 2011
Department of Chemistry, University of California, Irvine, California 92697-2025, USA.
In this Forum Article, we discuss the use of redox-active pincer-type ligands to enable multielectron reactivity, specifically nitrene group transfer, at the electron-poor metals tantalum and zirconium. Two analogous ligand platforms, [ONO] and [NNN], are discussed with a detailed examination of their similarities and differences and the structural and electronic constraints they impose upon coordination to early transition metals. The two-electron redox capabilities of these ligands enable the transfer of organic nitrenes to tantalum(V) and zirconium(IV) metal centers despite formal d(0) electron counts.
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