Nonlinear multiphoton absorption (MPA) upconversion lasers have critical applications in fluorescence imaging probes and biological photonics. Here, we report the realization of ultralow-threshold six-photon-excited upconversion lasing through cavity quantum electrodynamics effects in a plasmonic microcavity. The value of the Purcell factor () in hybrid whisper-gallery mode (WGM) is enhanced five-fold relative to a bare microwire (MW), which enhances the nonlinear light-matter interactions dramatically. Compared with a MW, the threshold of six-photon upconversion WGM lasing is reduced by one order magnitude due to plasmonic enhancement effects. In addition, the temperature and polarization characteristics of upconversion lasing a plasmonic-WGM approach show a distinct evolution, different from a bare MW. This work paves the way for extreme nonlinear optics, taking advantage of the processability and high Purcell factor of plasmonic microcavities.
Download full-text PDF |
Source |
|---|---|
| http://dx.doi.org/10.1039/d2nr01554d | DOI Listing |
Publication Analysis
Top Keywords
Similar Publications
Robust low threshold full-color upconversion lasing in rare-earth activated nanocrystal-in-glass microcavity.
Light Sci Appl
January 2025
State Key Laboratory of Luminescent Materials and Devices, and Guangdong Provincial Key Laboratory of Fiber Laser Materials and Applied Techniques, School of Materials Science and Engineering, South China University of Technology, 510640, Guangzhou, China.
Visible light microlasers are essential building blocks for integrated photonics. However, achieving low-threshold (μW), continuous-wave (CW) visible light lasing at room temperature (RT) has been a challenge because of the formidable requirement of population inversion at short wavelengths. Rare-earth (RE)-activated microcavities, featuring high-quality factor (Q) and small mode volume of whispering gallery modes, offer a great opportunity for achieving infrared-to-visible upconversion (UC) lasing.
View Article and Find Full Text PDFTwo-photon pumped forward, backward and random lasing in a stilbazolium dye nanocomposite solution containing LAPONITE® as a scattering center.
Nanoscale
December 2024
Department of Chemistry, University at Buffalo, SUNY, New York 14260, USA.
Multiphoton upconversion lasing in scattering gain media has attracted considerable attention in recent years. LAPONITE® is a scattering medium consisting of 2-D nano-discs that can be dispersed as a transparent solution in aqueous media and forms a gel at high concentration. In this paper, we demonstrate two-photon pumped upconversion regular lasing along forward and backward directions as well as random lasing along all other directions.
View Article and Find Full Text PDFIn this paper, fiber Bragg gratings (FBGs) are inscribed in Tm-doped fluorotellurite glass fiber (TDFTF) and applied to construction of a 2.3-µm all-fiber laser. The FBGs with a center wavelength of 2.
View Article and Find Full Text PDFUltrastable and Low-Threshold Two-Photon-Pumped Amplified Spontaneous Emission from CsPbBr/Ag Hybrid Microcavity.
Nanomaterials (Basel)
October 2024
School of Material Science and Engineering, Hanshan Normal University, Chaozhou 521041, China.
Halide perovskite materials have garnered significant research attention due to their remarkable performance in both photoharvesting photovoltaics and photoemission applications. Recently, self-assembled CsPbBr superstructures (SSs) have been demonstrated to be promising lasing materials. In this study, we report the ultrastable two-photon-pumped amplified stimulated emission from a CsPbBr SS/Ag hybrid microcavity with a low threshold of 0.
View Article and Find Full Text PDFIn this paper, we provide a new experimental insight into the lasing process in the erbium-doped tellurite glass fiber at high diode-pump powers and pumping pulse durations. It is shown that lasing occurs at two wavelengths. Initially, at a fixed wavelength of 2.
View Article and Find Full Text PDFWant AI Summaries of new PubMed Abstracts delivered to your In-box?
Enter search terms and have AI summaries delivered each week - change queries or unsubscribe any time!