Lutetium-yttrium oxyorthosilicate doped with cerium (LYSO:Ce) is a widely used scintillator, and the study of its nonlinear behavior under high excitation density is very significant owing to its direct influence on radiation measurements. Using a 266 nm ultraviolet laser to excite an LYSO:Ce crystal, the relationship between the photoluminescence (PL) light yield and excitation density was studied by scan experiments. The excitation threshold of the LYSO:Ce was obtained, which is about 2.3 J cm. Picosecond transient absorption of LYSO:Ce at 800 nm was obtained and used to analyze the dynamic process of carriers. The physical mechanism behind the nonlinearity was discussed and analyzed using the Förster dipole-dipole interaction model, and the interaction characteristic radius was obtained by fitting. This work can help us understand the nonlinearity phenomenon in scintillators and provide references for related radiation detection applications.
Download full-text PDF |
Source |
|---|---|
| http://www.ncbi.nlm.nih.gov/pmc/articles/PMC9031501 | PMC |
| http://dx.doi.org/10.1039/d1ra00347j | DOI Listing |
Publication Analysis
Top Keywords
Similar Publications
Spatiotemporal observation of surface plasmon polariton mediated ultrafast demagnetization.
Nat Commun
January 2025
School of Engineering Sciences, KTH Royal Institute of Technology, Applied Physics, AlbaNova, SE-106 91, Stockholm, Sweden.
Surface plasmons offer a promising avenue in the pursuit of swift and localized manipulation of magnetism for advanced magnetic storage and information processing technology. However, observing and understanding spatiotemporal interactions between surface plasmons and spins remains challenging, hindering optimal optical control of magnetism. Here, we demonstrate the spatiotemporal observation of patterned ultrafast demagnetization dynamics in permalloy mediated by propagating surface plasmon polaritons with sub-picosecond time- and sub-μm spatial- scales by employing Lorentz ultrafast electron microscopy combined with excitation through transient optical gratings.
View Article and Find Full Text PDFQuantum magnetometry of transient signals with a time resolution of 1.1 nanoseconds.
Nat Commun
January 2025
Department of Physics, ETH Zürich, Otto-Stern-Weg 1, 8093, Zürich, Switzerland.
Quantum magnetometers based on spin defects in solids enable sensitive imaging of various magnetic phenomena, such as ferro- and antiferromagnetism, superconductivity, and current-induced fields. Existing protocols primarily focus on static fields or narrow-band dynamical signals, and are optimized for high sensitivity rather than fast time resolution. Here, we report detection of fast signal transients, providing a perspective for investigating the rich dynamics of magnetic systems.
View Article and Find Full Text PDFInsights Into the Local Heating Effects in Triple-Cation Mixed-Halide Perovskite Cells: Charge Dynamics, Coherent Phonons, Anion Segregation.
Small
January 2025
Faculty of Physics and Astronomy, Adam Mickiewicz University, Poznan, 61-614, Poland.
The behavior of triple-cation mixed halide perovskite solar cells (PSCs) under ultrashort laser pulse irradiation at varying fluences is investigated, with a focus on local heating effects observed in femtosecond transient absorption (TA) studies. The carrier cooling time constant is found to increase from 230 fs at 2 µJ cm⁻ to 1.3 ps at 2 mJ cm⁻ while the charge population decay accelerates from tens of nanoseconds to the picosecond range within the same fluence range.
View Article and Find Full Text PDFDecoupling Carrier Dynamics and Energy Transport in Ultrafast Near-Field Nanoscopy.
Nano Lett
January 2025
Laser Thermal Laboratory, Department of Mechanical Engineering, University of California, Berkeley, California 94720, United States.
Ultrafast near-field optical nanoscopy has emerged as a powerful platform to characterize low-dimensional materials. While analytical and numerical models have been established to account for photoexcited carrier dynamics, quantitative evaluation of the associated pulsed laser heating remains elusive. Here, we decouple the photocarrier density and temperature increase in near-field nanoscopy by integrating the two-temperature model (TTM) with finite-difference time-domain (FDTD) simulations.
View Article and Find Full Text PDFMechanism of Amplified Photoacoustic Effect for Silica-Coated Spherical Gold Nanoparticles.
Nano Lett
January 2025
Department of Mechanical Engineering, the University of Texas at Dallas, Richardson, Texas 75080, United States.
Plasmonic nanomaterials are effective photoacoustic (PA) contrast agents with diverse biomedical applications. While silica coatings on gold nanoparticles (AuNPs) have been demonstrated to increase PA efficiency, the underlying mechanism remains elusive. Here, we systematically investigated the impact of silica coatings on PA generation under picosecond and nanosecond laser pulses.
View Article and Find Full Text PDFWant AI Summaries of new PubMed Abstracts delivered to your In-box?
Enter search terms and have AI summaries delivered each week - change queries or unsubscribe any time!