In this work, we report the modification of commercially available electrochemical electrodes with tin oxide (SnO) and Pd doped SnO (Pd-SnO) via pulsed laser-induced forward transfer (LIFT). The pulsed light irradiation working as in situ pulsed photo-thermal treatment allows for the transfer of SnO and Pd-SnO from UV absorbing metal complex precursors onto flexible, commercially available screen-printed electrodes. The laser transfer conditions are optimized and the material transferred under different conditions is evaluated morphologically and chemically, and its functionality is tested against the detection of copper ions. For example, by applying laser fluences in the range 100-250 mJ/cm, the shape and the size of the transferred features ranges from nano-polyhedrons to near corner-grown cubic Pd-SnO or near cubic Pd-SnO. In addition, the EDX analysis is consistent with the XPS findings, i.e., following laser transfer, Pd amounts lower than 0.5% are present in the Pd-SnO pixels. First sensing tests were carried out and the transferred Pd-SnO proved to enhance the cathodic peak when exposed to Cu(II) ions. This photo-initiated fabrication technology opens a promising way for the low-cost and high-throughput manufacturing of metal oxides as well as for electrodes for heavy metal ion detection.
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http://dx.doi.org/10.3390/ma15072488 | DOI Listing |
J Morphol
January 2025
Department of Zoology, Denver Museum of Nature & Science, Denver, Colorado, USA.
The barn owl is a common research subject in auditory science due to its exceptional capacity for high frequency hearing and superb sound source localization capabilities. Despite longstanding interest in the auditory performance of barn owls, the function of its middle ear has attracted remarkably little attention. Here, we report the middle ear transfer function measured by laser Doppler vibrometry and direct measurements of inner ear pressures.
View Article and Find Full Text PDFPhys Rev Lett
December 2024
Lawrence Berkeley National Laboratory, Berkeley, California 94720, USA.
We measure the high-intensity laser propagation throughout meter-scale, channel-guided laser-plasma accelerators by adjusting the length of the plasma channel on a shot-by-shot basis, showing high-quality guiding of 500 TW laser pulses over 30 cm in a hydrogen plasma of density n_{0}≈1×10^{17} cm^{-3}. We observed transverse energy transport of higher-order modes in the first ≈12 cm of the plasma channel, followed by quasimatched propagation, and the gradual, dark-current-free depletion of laser energy to the wake. We quantify the laser-to-wake transfer efficiency limitations of currently available petawatt-class lasers and demonstrate via simulation how control over the laser mode can significantly improve beam parameters.
View Article and Find Full Text PDFPhys Rev Lett
December 2024
Department of Physics, Durham University, South Road, Durham DH1 3LE, United Kingdom.
Many experimental platforms for quantum science depend on state control via laser fields. Frequently, however, the control fidelity is limited by optical phase noise. This is exacerbated in stabilized laser systems where high-frequency phase noise is an unavoidable consequence of feedback.
View Article and Find Full Text PDFNano Lett
January 2025
State Key Laboratory for Mesoscopic Physics and Frontiers Science Center for Nano-optoelectronics, School of Physics, Peking University, 100871 Beijing, China.
Strong coupling between nanocavities and single excitons at room temperature is important for studying cavity quantum electrodynamics. However, the coupling strength is highly dependent on the spatial light-confinement ability of the cavity, the number of involved excitons, and the orientation of the electric field within the cavity. By constructing a hybrid cavity with a one-dimensional photonic crystal cavity and a plasmonic nanocavity, we effectively improve the quality factor, reduce the mode volume, and control the direction of the electric field using Bloch surface waves.
View Article and Find Full Text PDFAlzheimers Dement
December 2024
The Miami Project to Cure Paralysis, Miami, FL, USA.
Background: Stroke and AD patients with gut complications often present worsened neurological outcomes. The goal of this study was to examine the role of extracellular vesicle (EV)-mediated pyroptosis in the bi-directional gut-brain axis after photothrombotic stroke (PTS) in aged 3xTg mice and wildtype (WT) controls.
Method: Twelve-month 3xTg and WT male and female mice underwent PTS using a YAG laser.
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