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Coupling Bifunctional Scaffolds with Slow Photon Effect for Synergistically Enhanced Photoassisted Lithium-Sulfur Battery Properties.
ACS Nano
January 2025
Institute of Flexible Electronics, Xi'an Key Laboratory of Flexible Electronics, Northwestern Polytechnical University, Xi'an 710072, China.
Photoassisted lithium-sulfur (Li-S) batteries offer a promising approach to enhance the catalytic transformation kinetics of polysulfide. However, the development is greatly hindered by inadequate photo absorption and severe photoexcited carriers recombination. Herein, a photonic crystal sulfide heterojunction structure is designed as a bifunctional electrode scaffold for photoassisted Li-S batteries.
View Article and Find Full Text PDFFrustrated Lewis Pair Meets Polyhedral Oligomeric Silsesquioxane: Water-Tolerant Hybrid Porous Networks for Robust, Efficient, and Recyclable CO Catalysis.
ACS Appl Mater Interfaces
January 2025
State Key Laboratory of Molecular Engineering of Polymers, Fudan University, Shanghai 200433, China.
Frustrated Lewis pair chemistry (FLP) occupy a crucial position in nonmetal-mediated catalysis, especially toward activation of inert gas molecules. Yet, one formidable issue of homogeneous FLP catalysts is their instability on preservation and recycling. Here we contribute a general solution that marries the polyhedral oligomeric silsesquioxane (POSS) with a structurally specific frustrated Lewis acid to fabricate porous polymer networks, which can form water-insensitive heterogeneous FLP catalysts upon employing Lewis base substrates.
View Article and Find Full Text PDFPoly(amic acid)-Polyimide Copolymer Interfacial Layers for Self-Powered CHNHPbI Photovoltaic Photodiodes.
Polymers (Basel)
January 2025
Department of Electrical and Biological Physics, Kwangwoon University, Wolgye-Dong, Seoul 01897, Republic of Korea.
Hybrid organohalide perovskites have received considerable attention due to their exceptional photovoltaic (PV) conversion efficiencies in optoelectronic devices. In this study, we report the development of a highly sensitive, self-powered perovskite-based photovoltaic photodiode (PVPD) fabricated by incorporating a poly(amic acid)-polyimide (PAA-PI) copolymer as an interfacial layer between a methylammonium lead iodide (CHNHPbI, MAPbI) perovskite light-absorbing layer and a poly(3,4-ethylenedioxythiophene)-poly(styrene sulfonate) (PEDOT: PSS) hole injection layer. The PAA-PI interfacial layer effectively suppresses carrier recombination at the interfaces, resulting in a high power conversion efficiency () of 11.
View Article and Find Full Text PDFPorosity Tunable Metal-Organic Framework (MOF)-Based Composites for Energy Storage Applications: Recent Progress.
Polymers (Basel)
January 2025
Department of Physics, Faculty of Science, Kasetsart University, Bangkok 10900, Thailand.
To solve the energy crisis and environmental issues, it is essential to create effective and sustainable energy conversion and storage technologies. Traditional materials for energy conversion and storage however have several drawbacks, such as poor energy density and inadequate efficiency. The advantages of MOF-based materials, such as pristine MOFs, also known as porous coordination polymers, MOF composites, and their derivatives, over traditional materials, have been thoroughly investigated.
View Article and Find Full Text PDFAntistaphylococcal Triazole-Based Molecular Hybrids: Design, Synthesis and Activity.
Pharmaceuticals (Basel)
January 2025
Department of Microbiology, Virology and Immunology, I. Horbachevsky Ternopil State Medical University, 46001 Ternopil, Ukraine.
Background: In the era of resistance, the design and search for new "small" molecules with a narrow spectrum of activity that target a protein or enzyme specific to a certain bacterium with high selectivity and minimal side effects remains an urgent problem of medicinal chemistry. In this regard, we developed and successfully implemented a strategy for the search for new hybrid molecules, namely, the not broadly known [2-(3-R-1-[1,2,4]-triazol-5-yl)phenyl]amines. They can act as "building blocks" and allow for the introduction of certain structural motifs into the desired final products in order to enhance the antistaphylococcal effect.
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