Herein, we report a remotely controlled soft robot employing a photoresponsive nanocomposite synthesized from liquid crystal elastomers (LCEs), high elastic form-stable phase change polymer (HEPCP), and multiwalled carbon nanotubes (MWCNTs). Possessing a two-stage deformation upon exposure to near-infrared (NIR) light, the LCE/HEPCP/MWCNT (LHM) nanocomposite allows the soft robot to exhibit an obvious, fast, and reversible shape change with low detection limitations. In addition to the deformation and bending of the LCE molecular chains itself, the HEPCP in the composite material can also be triggered by a reversible solid-liquid transition due to the temperature rise caused by MWCNTs, which further promotes the change of the LCE. In particular, the proposed photodriven LHM soft robot can bend up to 180° in 2 s upon NIR stimulation (320 mW, distance of 5 cm) and generate recoverable, dramatic, and sensitive deformation to execute various tasks including walking, twisting, and bending. With the capacity of imitating biological behaviors through remote control, the disruptive innovation developed here offers a promising path toward miniaturized untethered robotic systems.
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