Polarization-based colour tuning of mixed colloidal quantum-dot thin films using direct patterning.

Nanoscale

Optical Materials Engineering Laboratory, ETH Zürich, Leonhardstrasse 21, Zürich 8092, Switzerland.

Published: March 2022

Colloidal quantum-dots (cQDs) are finding increasingly widespread application in photonics and optoelectronics, providing high brightness and record-wide colour gamuts. However, the external quantum efficiencies in thin-film device architectures are still limited due to losses into waveguide modes and different strategies are being explored to promote the outcoupling of emission. Here we use a template-stripping-based direct-patterning strategy to fabricate linear gratings at the surface of cQD thin films. The linear gratings enhance optical outcoupling through Bragg scattering, yielding bright emission with a strong degree of linear polarization. By patterning linear gratings with different periodicities and orientations onto a film of mixed-colour cQDs, we demonstrate polarization-based active colour tuning of the thin-film emission.

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Source
http://dx.doi.org/10.1039/d1nr07136jDOI Listing

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