The functionality of a nanoscale silicon-based optoelectronic modulator is deeply analyzed while it appears that two competing processes, thermal and photonic, are occurring at the same time, and are preventing the optimization of the electro-optics coupling. While an incident illumination-beam first process is translated into photons, generating pairs of electrons-holes, a second process of thermal generation, creating phonons enables a loss of energy. Complementary studies, combining strong analytical models and numerical simulations, enabled to better understand this competition between photonic and thermal activities, in order to optimize the modulator. Moreover, in order to prevent unnecessary heating effects and to present a proposed solution, a picosecond pulsed laser is suggested and demonstrated as the ultimate solution so no energy will be wasted in heat, and still the photonic energy will be fully used. First ever-analytical solution to the heating produced due to the laser illumination applied on a nano-photonic device, while the illumination is produced in a periodic time changing function, e.g. a pulsed illumination, is presented. The present case study and proposed adapted solution can serve as a basis of generic approach in sensors' activation towards optimized photonics absorption.
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http://dx.doi.org/10.1038/s41598-021-04710-w | DOI Listing |
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January 2025
Faculty of Physics and Astronomy, Adam Mickiewicz University, Poznan, 61-614, Poland.
The behavior of triple-cation mixed halide perovskite solar cells (PSCs) under ultrashort laser pulse irradiation at varying fluences is investigated, with a focus on local heating effects observed in femtosecond transient absorption (TA) studies. The carrier cooling time constant is found to increase from 230 fs at 2 µJ cm⁻ to 1.3 ps at 2 mJ cm⁻ while the charge population decay accelerates from tens of nanoseconds to the picosecond range within the same fluence range.
View Article and Find Full Text PDFAtoms in Rydberg states are an important building block for emerging quantum technologies. While excitation to Rydberg orbitals is typically achieved in more than tens of nanoseconds, the physical limit is in fact much faster, at the ten picoseconds level. Here, we tackle such ultrafast Rydberg excitation of a rubidium atom by designing a dedicated pulsed laser system generating 480 nm pulses of 10 ps duration.
View Article and Find Full Text PDFNano Lett
January 2025
Laser Thermal Laboratory, Department of Mechanical Engineering, University of California, Berkeley, California 94720, United States.
Ultrafast near-field optical nanoscopy has emerged as a powerful platform to characterize low-dimensional materials. While analytical and numerical models have been established to account for photoexcited carrier dynamics, quantitative evaluation of the associated pulsed laser heating remains elusive. Here, we decouple the photocarrier density and temperature increase in near-field nanoscopy by integrating the two-temperature model (TTM) with finite-difference time-domain (FDTD) simulations.
View Article and Find Full Text PDFNano Lett
January 2025
Department of Mechanical Engineering, the University of Texas at Dallas, Richardson, Texas 75080, United States.
Plasmonic nanomaterials are effective photoacoustic (PA) contrast agents with diverse biomedical applications. While silica coatings on gold nanoparticles (AuNPs) have been demonstrated to increase PA efficiency, the underlying mechanism remains elusive. Here, we systematically investigated the impact of silica coatings on PA generation under picosecond and nanosecond laser pulses.
View Article and Find Full Text PDFSci Rep
December 2024
Institute of Physics and Center for Interdisciplinary Nanostructure Science and Technology (CINSaT), University of Kassel, Heinrich-Plett-Strasse 40, 34132, Kassel, Germany.
The ultrafast ionic dynamics in solids induced by intense femtosecond laser excitation are controlled by two fundamentally different yet interrelated phenomena. First, the substantial generation of hot electron-hole pairs by the laser pulse modifies the interatomic bonding strength and characteristics, inducing nonthermal ionic motion. Second, incoherent electron-ion collisions facilitate thermal equilibration between electrons and ions, achieving a uniform temperature on a picosecond timescale.
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