The ability to manipulate and measure the time-frequency structure of quantum light is useful for information processing and metrology. Measuring this structure is also important when developing quantum light sources with high modal purity that can interfere with other independent sources. Here, we present and experimentally demonstrate a scheme based on intensity interferometry to measure the joint spectral mode of photon pairs produced by spontaneous parametric down-conversion. We observe correlations in the spectral phase of the photons due to chirp in the pump. We show that our scheme can be combined with stimulated emission tomography to quickly measure their mode using bright classical light. Our scheme does not require phase stability, nonlinearities, or spectral shaping and thus is an experimentally simple way of measuring the modal structure of quantum light.
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http://dx.doi.org/10.1103/PhysRevLett.128.023601 | DOI Listing |
Phys Chem Chem Phys
January 2025
LPHE-MS, Faculty of Science, Mohammed V University in Rabat, Morocco.
This study explores the optoelectronic and photovoltaic potential of acceptor-π-donor (A-π-D) architectures utilizing CSi quantum dots (CSiQDs) through a combination of density functional theory (DFT) and time-dependent DFT (TDDFT). We examined two key structural configurations: C-C and Si-C conformers. In these systems, CSiQDs serve as the acceptor, CHSF as the π-bridge, and 3 × (CHO) as the donor.
View Article and Find Full Text PDFHeliyon
January 2025
Department of Physics, Facility of Science, King Abdulaziz University, Jeddah, Saudi Arabia.
The influence of variations in indium concentration and temperature on threshold current density (J) in In Ga As/GaAs ( = 0, 0.8 and 0.16) quantum dot (QD) laser diodes - synthesized via molecular beam epitaxy (MBE) with three distinct indium concentrations on GaAs (001) substrates - was meticulously examined.
View Article and Find Full Text PDFHeliyon
January 2025
Department of Chemistry, An-Najah National University, Nablus, Palestine.
While CuS/TiO₂ has been previously synthesized and employed in a limited number of photodegradation studies, the current study investigated its effectiveness for TC degradation under UV-visible light irradiation. CuS is known to be a nontoxic, environmentally friendly material; hence, it has great potential as an alternative to CdS and CdSe, which are used conventionally as sensitizers. In this work, the CuS/TiO₂ photocatalysts achieved a maximum 95 % removal of TC at an initial concentration of 20 ppm, confirming the good utilization of active sites.
View Article and Find Full Text PDFOrg Lett
January 2025
Key Laboratory of Material Chemistry for Energy Conversion and Storage, Ministry of Education, School of Chemistry and Chemical Engineering, Huazhong University of Science and Technology, Wuhan 430074, China.
Hindered tetraphenylethylene (hTPE) helicates are resolved into two left-handed (M) and right-handed (P) isomers by linkage and removal of chiral auxiliary (1,2,5)-menthol, furnishing gram-scale hTPE enantiomers via flash silica column chromatography. hTPE helicate enantiomers bearing electron-accepting cyano and electron-donating triphenylamine groups can emit deep-blue CPL signals with a fluorescence quantum yield surpassing 50%. Full-color and white-light emission were achieved by blending them with dyes in a poly(methyl methacrylate) (PMMA) film.
View Article and Find Full Text PDFWave mixing (WM) techniques are crucial for applications such as supercontinuum generation, frequency conversion, and high-dimensional quantum encoding. However, their efficiency is often limited by complex phase-matching requirements, and current insights into phase-matching mechanisms for high-order WM remain limited. To address this, compact optical path configurations with high-peak-power, synchronous, multicolor ultrafast laser sources are needed to enhance high-order wave-mixing efficiency.
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