Solar water evaporation is universally considered as an effective method to alleviate the freshwater shortage worldwide. A series of three-dimensional, salt-resistant evaporators have been brought out to improve the evaporation performance. However, little attention was paid to the collection of salt from seawater and high salinity brine. In this work, a carbon black polyvinyl alcohol (PVA) sponge was prepared to harvest light using a physical adsorption method to load carbon black on the PVA sponge. The experimental results showed that optimal light absorption (97.8%) and evaporation rate (1.60 kg m h) were achieved when the carbon black PVA sponge was produced at a carbon black concentration of 1 g L. Moreover, we stacked PVA sponges beneath the carbon black PVA sponge to construct a non-photothermal evaporation area. It was seen that the evaporator with an eight-layer PVA sponge had an excellent evaporation rate as high as 2.35 kg m h. In addition, the salt-collecting paper, all-black printed by a laser printer, was inserted between the stacked PVA sponges for salt collection, and the eight-layer PVA sponge evaporator with the salt-collecting paper at the fourth floor was tested in a 2 h desalination experiment. The outcome indicated that a square meter of this evaporator can produce about 7.03 L of freshwater and 206 g of salt per day from 10 wt % NaCl solution. As a result, the solar evaporator developed in this work is capable of collecting salt and maintaining a high evaporation rate, which is of great competence in the fields of freshwater production and salt collection.
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http://dx.doi.org/10.1021/acsami.1c17534 | DOI Listing |
Langmuir
January 2025
Ningbo Key Lab of Polymer Materials, Ningbo Institute of Materials Technology and Engineering, Chinese Academy of Sciences, 315211 Ningbo, P. R. China.
Solar-driven desalination technology is currently an important way to obtain freshwater resources. Significantly, porous materials are used as substrate materials of interface solar evaporator, and their specific impact of water transport property and thermal management during evaporation is worth exploring. In this paper, poly(vinyl alcohol) (PVA) sponges were prepared by a chemical foaming method, adjusted the PVA polymerization degree, and formaldehyde-hydroxyl ratio to regulate the pore size, and polypyrrole (PPy) was grown in situ on the surface skeleton of PVA sponge to construct a new interfacial solar evaporator (PPy/PVA) with different pore structures.
View Article and Find Full Text PDFCarbohydr Polym
March 2025
School of Chemistry and Chemical Engineering, North University of China, NO. 3 Xueyuan Road, Jiancaoping District, Taiyuan 030051, China. Electronic address:
Superhydrophilic hydrogel was typically used as the membrane coating on various substrates for oil/water separation. Nevertheless, these coatings may suffer from such limitations as poor adhesion strength and abrasion-resistance. Thus, the facile construction of hydrogel sponge with 3D connecting channels would be an ideal choice.
View Article and Find Full Text PDFLangmuir
January 2025
Key Laboratory for Advanced Technology in Environmental Protection of Jiangsu Province, Yancheng Institute of Technology, Yancheng 224051, China.
Electrode materials with a deformation capability are vital to the development of flexible supercapacitors. However, the preparation of porous carbons with a deformability remains challenging. Herein, a compressible carbon foam has been successfully prepared using a polydopamine/melamine sponge (PDA/MS) as the precursor material.
View Article and Find Full Text PDFJ Hazard Mater
December 2024
Center for Membrane Separation and Water Science & Technology, College of Chemical Engineering, Zhejiang University of Technology, Hangzhou 310014, China.
Heatable super hydrophobic polyurethane (PU) sponges (S-GNS/CNT/PVA@PU) containing three-dimensional (3D) carbon nano-networks (CNNs) coatings made from two-dimensional (2D) expanded graphite nano-sheets (GNS) bridged by one-dimensional (1D) carbon nano-tubes (CNT) were constructed using polyvinyl alcohol (PVA) as binder, in which light and/or electric energy could be rapidly converted into heat to reduce the viscosity of spilled heavy oils, resulting in greatly increased oil. Their heavy oil recovery rate could reach 792 kg/(m·h) under combined light and Joule heating of 1 sun and 5 V. Surface heat dissipating coefficient Ks, heat dissipating index n, and surface heat absorption capacity Cs were studied relating to sizes and shapes of surface heating fields under varied heating modes.
View Article and Find Full Text PDFACS Nano
January 2025
School of Materials Science and Engineering, Nanyang Technological University, 50 Nanyang Avenue, Singapore 639798, Republic of Singapore.
Hydrogel-based sensors have been widely studied for perceiving the environment. However, the simplest type of resistive sensors still lacks sensitivity to localized strain and other extractable data. Enhancing their sensitivity and expanding their functionality to perceive multiple stimuli simultaneously are highly beneficial yet require optimal material design and proper testing methods.
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