Strong coupling between an inverse bowtie Nano-Antenna and a J-aggregate.

J Colloid Interface Sci

Department of Chemistry, Institute of Nanotechnology and Advanced Materials (BINA), Bar-Ilan University, Ramat-Gan 5290002, Israel. Electronic address:

Published: March 2022

We demonstrate strong coupling between a single or few J-aggregates and an inverse bowtie plasmonic structure, when the J-aggregate is located at a specific axial distance from the metallic surface. Three hybrid modes are clearly observed, witnessing a strong interaction, with a Rabi splitting of up to 290 meV, the precise value of which significantly depends on the orientation of the J-aggregate with respect to the symmetry axis of the plasmonic structure. We repeated our experiments with a set of triangular hole arrays, showing consistent formation of three or more hybrid modes, in good agreement with numerical simulations.

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http://dx.doi.org/10.1016/j.jcis.2021.12.061DOI Listing

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