Tuning Coherent-Phonon Heat Transport in LaCoO/SrTiO Superlattices.

J Phys Chem Lett

Centro Singular de Investigación en Química Biolóxica e Materiais Moleculares (CIQUS), Departamento de Química-Física, Universidade de Santiago de Compostela, 15782 Santiago de Compostela, Spain.

Published: December 2021

Accessing the regime of coherent phonon propagation in nanostructures opens enormous possibilities to control the thermal conductivity in energy harvesting devices, phononic circuits, etc. In this paper we show that coherent phonons contribute substantially to the thermal conductivity of LaCoO/SrTiO oxide superlattices, up to room temperature. We show that their contribution can be tuned through small variations of the superlattice periodicity, without changing the total superlattice thickness. Using this strategy, we tuned the thermal conductivity by 20% at room temperature. We also discuss the role of interface mixing and epitaxial relaxation as an extrinsic, material dependent key parameter for understanding the thermal conductivity of oxide superlattices.

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Source
http://www.ncbi.nlm.nih.gov/pmc/articles/PMC8686111PMC
http://dx.doi.org/10.1021/acs.jpclett.1c03418DOI Listing

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