Direct Observation of Collective Electronuclear Modes about a Quantum Critical Point.

Phys Rev Lett

Division of Physics, Mathematics, and Astronomy, California Institute of Technology, Pasadena, California 91125, USA.

Published: November 2021

We directly measure the low energy excitation modes of the quantum Ising magnet LiHoF_{4} using microwave spectroscopy. Instead of a single electronic mode, we find a set of collective electronuclear modes, in which the spin-1/2 Ising electronic spins hybridize with the bath of spin-7/2 Ho nuclear spins. The lowest-lying electronuclear mode softens at the approach to the quantum critical point, even in the presence of disorder. This softening is rapidly quenched by a longitudinal magnetic field. Similar electronuclear structures should exist in other spin-based quantum Ising systems.

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http://dx.doi.org/10.1103/PhysRevLett.127.207202DOI Listing

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