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Room-Temperature All-Solid-State Sodium Battery Based on Bulk Interfacial Superionic Conductor. | LitMetric

Room-Temperature All-Solid-State Sodium Battery Based on Bulk Interfacial Superionic Conductor.

Nano Lett

School of Chemistry and Chemical Engineering, Frontiers Science Center for Transformative Molecules, and in situ Center for Physical Sciences, Shanghai Jiao Tong University, Shanghai 200240, P.R. China.

Published: December 2021

AI Article Synopsis

Article Abstract

All-solid-state sodium batteries (ASSSBs) are attractive alternatives to lithium-ion batteries for grid-scale energy storage due to their high safety and ubiquitous distribution of Na sources. A critical component for ASSSB is sodium-ion conducting solid-state electrolyte (SSE). Here, we report a high-performance sodium-ion SSE with the recently developed bulk interfacial superionic conductor (BISC) concept. The ionic conductivity and areal conductance of the Na BISC at 25 °C reaches 6.5 × 10 S cm and 260 mS cm, respectively. Using NaCoMnO ( ≈ 1.0, NaCMO) as the cathode active material, all-solid-state Na||NaCMO batteries exhibiting small overpotential and ∼180 cycle life are demonstrated under room temperature. This approach may also be used to prepare other metal ion, such as Mg, Al, and K, based all-solid-state batteries.

Download full-text PDF

Source
http://dx.doi.org/10.1021/acs.nanolett.1c03605DOI Listing

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