A large anomalous Nernst effect (ANE) is crucial for thermoelectric energy conversion applications because the associated unique transverse geometry facilitates module fabrication. Topological ferromagnets with large Berry curvatures show large ANEs; however, they face drawbacks such as strong magnetic disturbances and low mobility due to high magnetization. Herein, we demonstrate that YbMnBi, a canted antiferromagnet, has a large ANE conductivity of ~10 A m K that surpasses large values observed in other ferromagnets (3-5 A m K). The canted spin structure of Mn guarantees a non-zero Berry curvature, but generates only a weak magnetization three orders of magnitude lower than that of general ferromagnets. The heavy Bi with a large spin-orbit coupling enables a large ANE and low thermal conductivity, whereas its highly dispersive p orbitals ensure low resistivity. The high anomalous transverse thermoelectric performance and extremely small magnetization make YbMnBi an excellent candidate for transverse thermoelectrics.
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http://www.ncbi.nlm.nih.gov/pmc/articles/PMC8810386 | PMC |
http://dx.doi.org/10.1038/s41563-021-01149-2 | DOI Listing |
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