China is the largest iron and steel producer and consumer in the world. The iron and steel manufacture, especially the sintering process, is energy-intensive, and contributes substantially to air pollutant emissions in China. Compared with other regions, the Fenwei Plain, a coal base, has a heavy industry concentration, and high pollutant emission total amount. In addition, urban air pollution has rebounded, and the pollutants concentrations in many cities have increased rather than decreased. In this study, we investigated the inter-annual trends of particulate matter (PM), sulfur dioxide (SO) and nitrogen oxide (NO) from the sintering process of iron and steel industry (ISI) in the Fenwei Plain and the surrounding regions in China from 2014 to 2017 based on the Continuous Emission Monitoring System (CEMS). We found that the oxygen content of the flue gas is the key to judge whether the sintering flue gas air pollutant emission concentration can meet the standard. Therefore, we adopted the converted concentration by the reference oxygen content in the final analysis. Overall, the SO and PM emission concentrations exhibit a downward trend from 2014 to 2017, in response to the strengthening of the emission control policies and standards in the ISI, whereas the NO emission concentration did not change significantly during the same period The emission factors (EFs) of PM, NO and SO obtained in this study are lower than previous estimates. In 2017, the SO and PM emissions were 27% and 32% lower than the levels in 2014.While NO was 22% higher than the level in 2014. Our study confirmed the effectiveness of current emission control policies and standards in the iron and steel sector. However, the levels of NO emissions were still high until 2017, illustrating the urgent need for more advanced emission control technologies to further reduce NO emissions from the sintering flue gas in China.
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http://dx.doi.org/10.1016/j.chemosphere.2021.132917 | DOI Listing |
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