We report the generation of multiple sets of 3D confined resonant modes in a single microtube cavity owing to nanogap induced resonant trajectory splits. The optical field largely overlaps in the split resonant trajectories, enabling strong optical coupling of 3D confined resonant light. The anticrossing feature and modes changing-over were demonstrated as direct evidence of strong coupling. In such an optical coupling system, the spatial optical field distribution of 3D coupling modes was experimentally mapped under the strong coupling regime, which allows direct observation of the energy transfer process between two hybrid states. Numerical calculations based on a quasi-potential model and the mode detuning process are in excellent agreement with the experimental results. The generation of multiple sets of 3D confined resonant modes and their efficient coupling in a single microcavity are of high interest for directional coupling with a higher degree of freedom to realize on-chip integration with elevated functionalities such as multiplexing, 3D lasing, and signal processing.
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http://dx.doi.org/10.1021/acsnano.1c07968 | DOI Listing |
Nano Lett
January 2025
CAS Key Laboratory of Standardization and Measurement for Nanotechnology, National Center for Nanoscience and Technology, Beijing 100190, People's Republic of China.
Exciton emitters in two-dimensional monolayer transition-metal dichalcogenides (TMDs) provide a boulevard for the emerging optoelectronic field, ranging from miniaturized light-emitting diodes to quantum emitters and optical communications. However, the low quantum efficiency from limited light-matter interactions and harmful substrate effects seriously hinders their applications. In this work, we achieve a ∼438-fold exciton photoluminescence enhancement by constructing a Fabry-Pérot cavity consisting of monolayer WS and a micron-scale hole on the SiO/Si substrate.
View Article and Find Full Text PDFJ Biomed Opt
January 2025
TU Dresden, Carl Gustav Carus Faculty of Medicine, Anesthesiology and Intensive Care Medicine, Clinical Sensing and Monitoring, Dresden, Germany.
Significance: The precise identification and preservation of functional brain areas during neurosurgery are crucial for optimizing surgical outcomes and minimizing postoperative deficits. Intraoperative imaging plays a vital role in this context, offering insights that guide surgeons in protecting critical cortical regions.
Aim: We aim to evaluate and compare the efficacy of intraoperative thermal imaging (ITI) and intraoperative optical imaging (IOI) in detecting the primary somatosensory cortex, providing a detailed assessment of their potential integration into surgical practice.
Anal Bioanal Chem
January 2025
Turkish Petroleum Refineries Co. TÜPRAŞ R&D Center, Körfez, Kocaeli, 41790, Türkiye.
Monoelemental calibration solutions are the most common reference in elemental analysis, linking measurement results to the International System of Units (SI). National Metrology Institutes (NMI) prepare these solutions as certified reference materials (CRM) and determine their elemental mass fraction with high accuracy. Characterization with high accuracy is one of the most critical steps in CRM production.
View Article and Find Full Text PDFNat Chem
January 2025
Department of Chemistry, University of California Irvine, Irvine, CA, USA.
Controlling reaction outcomes through external influences is a central goal in chemistry. Vibrational coupling between molecular vibrations and cavity modes is rapidly emerging as a distinct strategy compared with conventional thermochemical and photochemical methods; however, insight into the fundamental mechanisms remains limited. Here we investigate how vibrational weak and strong coupling in plasmonic nanocavities modifies the thermal dehydration of copper sulfate pentahydrate.
View Article and Find Full Text PDFAnal Bioanal Chem
January 2025
Bio-analytical Laboratory, Shantou University Medical College, No. 22, Xinling Road, Shantou, 515041, China.
A polarimeter is a common but critical instrument for measuring the optical rotation of chiral compounds, ranging from the pharmaceutical to chemical industry, or even employed in monitoring chemical reactions for research purposes. Developing a portable polarimeter helps to transfer the measurements from the laboratory to on-site detection. Herein, we design a new portable polarimeter with a "hand-held" scale.
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