In this research, a highly sensitive and selective hydrogen gas sensor was developed based on Cu-doped SnO. Sensing characteristics were compared based on SnO doped with different concentrations of Cu, and the highest sensitivity and fastest response time were shown when 3% Cu was contained. A 3D structure was formed using a polystyrene to increase the surface-to-volume ratio, which allows more oxygen molecules to bond with the surface of the SnO sensing material. Extremely increased sensitivity was observed as compared to the planar structure. A temperature sensor and micro-heater were integrated into the sensor, and the surface temperature was maintained constant regardless of external influences. In addition, an electronic sensor interface was developed for the efficient analysis of real-time data. The developed sensor was wire-bonded to the flexible printed circuit board (FPCB) cable and connected with the sensor interface. Sensitivity and linearity measured based on the developed sensor and interface system were analyzed as 0.286%/ppm and 0.98, respectively, which were almost similar to the results observed by a digital multimeter (DMM). This indicates that our developed sensor system can be a very promising candidate for real-time measurement and can be applied in various fields. The enhanced sensitivity of 3% doped SnO toward hydrogen is attributed to the huge number of oxygen vacancies in the doped sample.
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http://dx.doi.org/10.1021/acssensors.1c01696 | DOI Listing |
ACS Nano
January 2025
State Key Laboratory of Flexible Electronics (LoFE) & Institute of Advanced Materials (IAM), School of Flexible Electronics (Future Technologies), Nanjing Tech University (Nanjing Tech), 30 South Puzhu Road, Nanjing 211816, China.
Neuromorphic vision sensors capable of multispectral perception and efficient recognition are highly desirable for bioretina emulation, but their realization is challenging. Here, we present a cocrystal strategy for preparing an organic nanowire retinamorphic vision sensor with UV-vis-NIR perception and fast recognition. By leveraging molecular-scale donor-acceptor interpenetration and charge-transfer interfaces, the cocrystal nanowire device exhibits ultrawide photoperception ranging from 350 to 1050 nm, fast photoresponse of 150 ms, high specific detectivity of 8.
View Article and Find Full Text PDFNano Lett
January 2025
School of Physical Science and Technology, ShanghaiTech University, 393 Middle Huaxia Road, Shanghai 201210, China.
Transpiration-driven electrokinetic power generators (TEPGs) hold promising potential for intelligent chemical sensing applications, enabling the efficient identification and screening of organic solvents. Here, we report a novel TEPG-based chemical sensor using MoS-doped cellulose filter paper for efficient detection of poplar solvents like water, alcohols, and methanol. TEPGs operate by leveraging capillary-driven transpiration to induce solvent flow through porous materials, leading to ion migration and the formation of electrical double layers (EDLs) at the solid-liquid interfaces.
View Article and Find Full Text PDFInt J Biol Macromol
January 2025
Department of Analytical Chemistry, Faculty of Chemistry, Razi University, Kermanshah, Iran.
This study introduces the development of a highly sensitive label-free electrochemical immunosensor specifically designed to detect prostate-specific antigen (PSA). A glassy carbon electrode (GCE) coated with Au nanoparticles/polyhedral hollow CoCu bimetallic sulfide (CuCoS) was employed as a sensing interface for the fixation of the monoclonal anti-PSA antibody. The nanoarchitectures enhanced the capacity for loading prostate-specific antibodies (Ab) and effectually boosted electrical conductivity leading to enhance the electrochemical signal and greater sensitivity for the detection of PSA.
View Article and Find Full Text PDFAnal Biochem
January 2025
Department of Biotechnology, National Institute of Pharmaceutical Education and Research, Sector 67, S.A.S. Nagar, Punjab 160062, India. Electronic address:
Aptamers, discovered in the 1990s, have marked a significant milestone in the fields of therapeutics and diagnostics. This review provides a comprehensive survey of aptamers, focusing on their diagnostic applications. It especially encapsulates a decade of aptamer, encompassing research, patents, and market trends.
View Article and Find Full Text PDFProc Natl Acad Sci U S A
February 2025
SKKU Advanced Institute of Nanotechnology (SAINT), Sungkyunkwan University, Suwon 16419, Republic of Korea.
The design of organic-peptide hybrids has the potential to combine our vast knowledge of protein design with small molecule engineering to create hybrid structures with complex functions. Here, we describe the computational design of a photoswitchable Ca-binding organic-peptide hybrid. The designed molecule, designated Ca-binding switch (CaBS), combines an EF-hand motif from classical Ca-binding proteins such as calmodulin with a photoswitchable group that can be reversibly isomerized between a spiropyran (SP) and merocyanine (MC) state in response to different wavelengths of light.
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