AI Article Synopsis
- Atomically thin materials (ATMs) are less than 5 nm thick and are ideal for creating high-performance electrode materials for various rechargeable batteries due to their large surface areas and strong chemical bonds.
- This work reviews the synthesis and tuning of the electronic properties of different ATMs, such as graphene, phosphorene, and MXenes, highlighting their potential for high-energy and high-power density batteries.
- The paper also discusses future challenges and opportunities in the development of efficient ATMs for advanced rechargeable battery technologies, critical for the growth of portable electronics and electric vehicles.
Article Abstract
Atomically thin materials (ATMs) with thicknesses in the atomic scale (typically <5 nm) offer inherent advantages of large specific surface areas, proper crystal lattice distortion, abundant surface dangling bonds, and strong in-plane chemical bonds, making them ideal 2D platforms to construct high-performance electrode materials for rechargeable metal-ion batteries, metal-sulfur batteries, and metal-air batteries. This work reviews the synthesis and electronic property tuning of state-of-the-art ATMs, including graphene and graphene derivatives (GE/GO/rGO), graphitic carbon nitride (g-CN), phosphorene, covalent organic frameworks (COFs), layered transition metal dichalcogenides (TMDs), transition metal carbides, carbonitrides, and nitrides (MXenes), transition metal oxides (TMOs), and metal-organic frameworks (MOFs) for constructing next-generation high-energy-density and high-power-density rechargeable batteries to meet the needs of the rapid developments in portable electronics, electric vehicles, and smart electricity grids. We also present our viewpoints on future challenges and opportunities of constructing efficient ATMs for next-generation rechargeable batteries.
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| http://dx.doi.org/10.1021/acs.chemrev.1c00636 | DOI Listing |
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