Gas-liquid interfaces (GLIs) are ubiquitous and have found widespread applications in a large variety of fields. Despite the recent trend of downscaling GLIs, their nanoscale fabrication remains challenging because of the lack of suitable tools. In this study, a nanofluidic device, which has undergone precise local surface modification, is used in combination with tailored physicochemical effects in nanospace and optimized nanofluidic operations, to produce uniform, arrayable, stable, and transportable nanoscale GLIs that can concentrate molecules of interest at the nanoscale. This approach provides a delicate nanofluidic mechanism for downscaling gas-liquid interfaces to the nanometer scale, thus opening up a new avenue for gas-liquid interface studies and applications.
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http://dx.doi.org/10.1021/acs.nanolett.1c02871 | DOI Listing |
Foods
December 2024
College of Food Science, Fujian Agriculture and Forestry University, Fuzhou 350002, China.
Soy protein isolate (SPI) possesses potential gelling properties, making it suitable for gel-based applications. However, the gel network stability and mechanical properties of SPI are relatively poor and can be improved through modifications or by combining it with other polymers, such as Konjac Glucomannan (KGM). Combining SPI with KGM can overcome the poor gel network stability and mechanical properties of SPI, but it reduces the water-absorbing capacity of the gel network after drying, which affects the quality characteristics of plant-based protein rehydrated foods and limits the economic feasibility of soy protein foods.
View Article and Find Full Text PDFEnviron Sci Technol
January 2025
Zhejiang Key Laboratory of Clean Energy Conversion and Utilization, Science and Education Integration College of Energy and Carbon Neutralization, Zhejiang University of Technology, Hangzhou 310014, China.
ACS Meas Sci Au
December 2024
Department of Chemistry, The University of Texas at Austin, Austin, Texas 78712, United States.
The gas-liquid-solid interface plays a crucial role in various electrochemical energy conversion devices, including fuel cells and electrolyzers. Understanding the effect of gas transfer on the electrochemistry at this three-phase interface is a grand challenge. Scanning electrochemical cell microscopy (SECCM) is an emerging technique for mapping the heterogeneity in electrochemical activity; it also inherently features a three-phase boundary at the nanodroplet cell.
View Article and Find Full Text PDFSci Total Environ
December 2024
Key Laboratory of Ocean Energy Utilization and Energy Conservation of Ministry of Education, Dalian University of Technology, Dalian 116024, China. Electronic address:
Marine carbon sequestration, with its high potential and low risk of leakage, is an attractive technology for effectively addressing global climate change and reducing greenhouse gas emissions. A current concern about marine sequestration lies in the potential negative effects of the carbon sequestration process on the marine environment. CO hydrate sequestration is considered to be one of the most stable method of sequestration, and researchers are actively searching for promoters that facilitate hydrate sequestration and are friendly to the marine environment.
View Article and Find Full Text PDFACS Appl Mater Interfaces
December 2024
Key Laboratory of Bio-inspired Materials and Interfaces Sciences, Technical Institute of Physics and Chemistry, Chinese Academy of Sciences, Beijing 100190, China.
Azobenzene actuators have generated extensive research investment in the field of soft robots, artificial muscles, etc., based on the typical photoresponsive - isomerization. However, it remains challenging to achieve multiphase actuation at the gas-liquid interface and liquid phase.
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