Clusters and nanodroplets hold the promise of enhancing high-order nonlinear optical effects due to their high local density. However, only moderate enhancement has been demonstrated to date. Here, we report the observation of energetic electrons generated by above-threshold ionization (ATI) of helium (He) nanodroplets which are resonantly excited by ultrashort extreme ultraviolet (XUV) free-electron laser pulses and subsequently ionized by near-infrared (NIR) or near-ultraviolet (UV) pulses. The electron emission due to high-order ATI is enhanced by several orders of magnitude compared with He atoms. The crucial dependence of the ATI intensities with the number of excitations in the droplets suggests a local collective enhancement effect.
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http://dx.doi.org/10.1103/PhysRevLett.127.093201 | DOI Listing |
J Chem Phys
January 2025
Department of Chemistry, Johns Hopkins University, Baltimore, Maryland 21218, USA.
Electronic spectra for OThF have been recorded using fluorescence excitation and two-photon resonantly enhanced ionization techniques. Multiple vibronic bands were observed in the 340-460 nm range. Dispersed fluorescence spectra provided ground state vibrational constants and evidence of extensive vibronic state mixing at higher excitation energies.
View Article and Find Full Text PDFNpj Nanophoton
November 2024
Dipartimento di Fisica, Sapienza Università di Roma, Roma, Italy.
Quantum state teleportation represents a pillar of quantum information and a milestone on the roadmap towards quantum networks with a large number of nodes. Successful photonic demonstrations of this protocol have been carried out employing different qubit encodings. However, demonstrations in the Fock basis encoding are challenging, due to the impossibility of generating a coherent superposition of vacuum-one photon states on a single mode with linear optics.
View Article and Find Full Text PDFPhys Rev Lett
November 2024
Institute for Quantum Science and Engineering, Department of Physics and Astronomy, Texas A&M University, College Station, Texas 77843, USA.
Phys Chem Chem Phys
November 2024
Rzhanov Institute of Semiconductor Physics, SB RAS, Novosibirsk, 630090, Russia.
Interaction of phonons with Dirac-like electronic states sets the fundamental limit of electron transport in topological insulators (TIs). Polarization-resolved and resonant Raman scattering of bulk and surface electronic excitation and vibrational modes in BiTe and BiSbTeSe (BSTS) thin films was investigated. At photon energies () of 1.
View Article and Find Full Text PDFThis study introduces what we believe is a novel approach to manipulating light in the mid-infrared spectrum through phonon-mediated metal-insulator-metal (MIM) cavities. Leveraging the unique interactions between resonantly excited electric and magnetic dipoles and phonons within silicon dioxide spacers, we have developed a technology different from traditional methods that rely on geometric modifications of nanostructures, offering a more versatile and effective means of tailoring light-matter interactions at the nanoscale. Our experimental results showcase the ability of these MIM cavities to perform multifunctional information encoding, display, and concealment with high precision.
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