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Theoretical Understanding of Photoluminescence and Singlet Oxygen Quantum Yields in a Few Halogenated Fluorescein Dyes.
Chem Asian J
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Department of Chemistry, Indian Institute of Technology Tirupati, Tirupati, A.P 517619, India.
Visible-light absorbing metal-free organic dyes are of increasing demand for various optoelectronic applications because of their great structure-function tunability through chemical means. Several dyes also show huge potential in triplet photosensitization, generating reactive singlet oxygen. Understanding the structure-property relationships of many well-known fluorescein dyes is of paramount importance in designing next-generation energy efficient dyes, which is currently limited.
View Article and Find Full Text PDFAsparagopsis taxiformis supplementation to mitigate enteric methane emissions in dairy cows - effects on performance and metabolism.
J Dairy Sci
January 2025
Department of Applied Animal Science & Welfare, Swedish University of Agricultural Sciences (SLU), Box 7024, 753 23 Uppsala, Sweden.
Methane emissions from ruminant digestion contribute significantly to global anthropogenic greenhouse gas emissions. Members of the phylum Rhodophyta (red algae), particularly Asparagopsis sp., have shown promising results in reducing methane emissions in ruminants, due to their high content of halogenated methane analog compounds.
View Article and Find Full Text PDFAssociation Between Serum Concentrations of (Certain) Metals and Type 2 Diabetes Mellitus.
J Clin Med
December 2024
Department of Correct, Clinical and Imaging Anatomy, Medical University of Lublin, Jaczewskiego 4, 20-090 Lublin, Poland.
The findings regarding trace element concentrations in patients diagnosed with type 2 diabetes and healthy controls are inconsistent, and therefore, we determined to gather them in the form of a review to further indicate the need for more advanced knowledge development. In our study, we reviewed articles and studies that involved the topics of micronutrient and metal associations with the occurrence and development of type 2 diabetes. We mainly included works regarding human-based studies, but with limited research results, animal-based research was also taken into account.
View Article and Find Full Text PDFSynthesis and Application of 1-[F]Fluoro-4-isothiocyanatobenzene for Radiofluorination of Peptides in Aqueous Medium.
J Org Chem
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Department of Radiology, Mayo Clinic, Rochester, Minnesota 55906, United States.
Conjugation of radiofluorinated prosthetic groups to primary amines of peptides in an aqueous medium is still considerably challenging. Herein, we report a one-pot cascade synthesis of 1-[F]fluoro-4-isothiocyanatobenzene ([F]), an isothiocyanate-functionalized prosthetic group for radiolabeling of various peptides in aqueous medium. The developed compound [F] was synthesized in >99% radiochemical purity with 22.
View Article and Find Full Text PDFBenchmark Ab Initio Mapping of the F + CHClI S2 and Proton-Abstraction Reactions.
J Phys Chem A
December 2024
MTA-SZTE Lendület "Momentum" Computational Reaction Dynamics Research Group, Interdisciplinary Excellence Centre and Department of Physical Chemistry and Materials Science, Institute of Chemistry, University of Szeged, Szeged H-6720, Hungary.
Article Synopsis
- The studies of gas-phase S2 reactions have enhanced our understanding of basic chemical processes and their mechanisms, providing deep insights into chemical dynamics.
- This research focuses on the reactions involving fluorine and CHClI, using advanced computational methods to explore different reaction pathways and their associated energies.
- Findings indicate that additional halogenation of CHY alters reaction dynamics, making certain reaction pathways more favorable and reducing the prominence of the classic backside attack mechanism in favor of other processes like halogen-bonded complex formation.
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