We describe how the out-of-plane dielectric polarizability of monolayer graphene influences the electrostatics of bilayer graphene-both Bernal (BLG) and twisted (tBLG). We compare the polarizability value computed using density functional theory with the output from previously published experimental data on the electrostatically controlled interlayer asymmetry potential in BLG and data on the on-layer density distribution in tBLG. We show that monolayers in tBLG are described well by polarizability α = 10.8 Å and effective out-of-plane dielectric susceptibility ϵ = 2.5, including their on-layer electron density distribution at zero magnetic field and the interlayer Landau level pinning at quantizing magnetic fields.
Download full-text PDF |
Source |
---|---|
http://www.ncbi.nlm.nih.gov/pmc/articles/PMC8361429 | PMC |
http://dx.doi.org/10.1021/acs.nanolett.1c02211 | DOI Listing |
Nano Lett
January 2025
Department of Engineering Mechanics, Zhejiang University, Hangzhou, 310027 Zhejiang, China.
Chiral vortices and their phase transition in ferroelectric/dielectric heterostructures have drawn significant attention in the field of condensed matter. However, the dynamical origin of the chiral phase transition from achiral to chiral polar vortices has remained elusive. Here, we develop a phase-field perturbation model and discover the softening of out-of-plane vibration mode of polar vortices in [(PbTiO)/(SrTiO)] superlattices at a critical epitaxial strain or temperature.
View Article and Find Full Text PDFJ Phys Condens Matter
January 2025
Institute of Nano Science and Technology, Knowledge City, Sector 81, Manauli, Mohali, Punjab 140306, India.
Two-dimensional (2D) materials hold great promise for the next-generation optoelectronics applications, many of which, including solar cell, rely on the efficient dissociation of exciton into free charge carriers. However, photoexcitation in atomically thin 2D semiconductors typically produces exciton with a binding energy of ∼500 meV, an order of magnitude larger than thermal energy at room temperature. This inefficient exciton dissociation can limit the efficiency of photovoltaics.
View Article and Find Full Text PDFNat Commun
January 2025
Department of Physics, Massachusetts Institute of Technology, Cambridge, MA, USA.
Applying long wavelength periodic potentials on quantum materials has recently been demonstrated to be a promising pathway for engineering novel quantum phases of matter. Here, we utilize twisted bilayer boron nitride (BN) as a moiré substrate for band structure engineering. Small-angle-twisted bilayer BN is endowed with periodically arranged up and down polar domains, which imprints a periodic electrostatic potential on a target two-dimensional (2D) material placed on top.
View Article and Find Full Text PDFSci Rep
January 2025
School of Optical-Electrical and Computer Engineering, University of Shanghai for Science and Technology, Shanghai, 200093, China.
In recent years, research on chiral bound states in the continuum (BIC) has surged, leading to the development of various chiral metasurfaces with narrow bandwidths by breaking of in-plane and out-of-plane symmetries. However, the ability to dynamically tune the working band remains relatively unexplored, which is valuable for chiral sensing applications. Optical phase-change materials, with tunable dielectric constants and switchable properties during phase transition, offer the potential for dynamic control of optical metasurfaces.
View Article and Find Full Text PDFNat Commun
December 2024
Department of Materials Science and NanoEngineering and the Rice Advanced Materials Institute, Rice University, Houston, TX, 77005, USA.
As the feature size of microelectronic circuits is scaling down to nanometer order, the increasing interconnect crosstalk, resistance-capacitance (RC) delay and power consumption can limit the chip performance and reliability. To address these challenges, new low-k dielectric (k < 2) materials need to be developed to replace current silicon dioxide (k = 3.9) or SiCOH, etc.
View Article and Find Full Text PDFEnter search terms and have AI summaries delivered each week - change queries or unsubscribe any time!