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Microscopic interactions and emerging elasticity in model soft particulate gels. | LitMetric

Microscopic interactions and emerging elasticity in model soft particulate gels.

J Phys Condens Matter

Department of Physics, Institute for Soft Matter Synthesis and Metrology, Georgetown University, 37th and O Streets, N.W., Washington, D.C. 20057, United States of America.

Published: August 2021

We discuss a class of models for particulate gels in which the particle contacts are described by an effective interaction combining a two-body attraction and a three-body angular repulsion. Using molecular dynamics, we show how varying the model parameters allows us to sample, for a given gelation protocol, a variety of gel morphologies. For a specific set of the model parameters, we identify the local elastic structures that get interlocked in the gel network. Using the analytical expression of their elastic energy from the microscopic interactions, we can estimate their contribution to the emergent elasticity of the gel and gain new insight into its origin.

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Source
http://dx.doi.org/10.1088/1361-648X/ac14f6DOI Listing

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